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Endless Dirac nodal lines in kagome-metal Ni3In2S2
npj Computational Materials ( IF 9.7 ) Pub Date : 2022-07-19 , DOI: 10.1038/s41524-022-00838-z
Tiantian Zhang , T. Yilmaz , E. Vescovo , H. X. Li , R. G. Moore , H. N. Lee , H. Miao , S. Murakami , M. A. McGuire

Topological semimetals are a frontier of quantum materials. In multiband electronic systems, topological band crossings can form closed curves, known as nodal lines. In the presence of spin–orbit coupling and/or symmetry-breaking operations, topological nodal lines can break into Dirac/Weyl nodes and give rise to interesting transport properties, such as the chiral anomaly and giant anomalous Hall effect. Recently, the time-reversal symmetry-breaking induced Weyl fermions are observed in a kagome-metal Co3Sn2S2, triggering interests in nodal-line excitations in multiband kagome systems. Here, using first-principles calculations and symmetry-based indicator theories, we find six endless nodal lines along the stacking direction of kagome layers and two nodal rings in the kagome plane in nonmagnetic Ni3In2S2. The linear dipsersive electronic structure, confirmed by angle-resolved photoemission spectroscopy, induces large magnetoresistance up to 2000% at 9 T. Our results establish a diverse topological landscape of multiband kagome metals.



中文翻译:

Kagome 金属 Ni3In2S2 中的无尽狄拉克节点线

拓扑半金属是量子材料的前沿。在多频带电子系统中,拓扑带交叉可以形成闭合曲线,称为节点线。在存在自旋轨道耦合和/或对称破缺操作的情况下,拓扑节点线可以突破 Dirac/Weyl 节点并产生有趣的传输特性,例如手性异常和巨大异常霍尔效应。最近,在kagome-metal Co 3 Sn 2 S 2中观察到时间反演对称破缺诱导的Weyl费米子,引发对多频带kagome系统中节点线激励的兴趣。在这里,利用第一性原理计算和基于对称性的指标理论,我们在非磁性Ni 3 In 2 S 2中发现了沿kagome层堆叠方向的六个无限节线和kagome平面中的两个节环。由角分辨光电子能谱证实的线性色散电子结构在 9 T 时诱导高达 2000% 的大磁阻。我们的结果建立了多波段 kagome 金属的多样化拓扑景观。

更新日期:2022-07-19
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