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Advances in the Key Metal-Based Catalysts for Efficient Electrochemical Conversion of CO2
ChemBioEng Reviews ( IF 4.8 ) Pub Date : 2022-06-27 , DOI: 10.1002/cben.202200005
Jidsucha Darayen 1 , Orawon Chailapakul 2, 3 , Piyasan Praserthdam 4, 5 , Joongjai Panpranot 4, 5 , Duangamol N. Tungasmita 3 , Yuttanant Boonyongmaneerat 6
Affiliation  

The electrochemical reduction process is one of the most promising approaches to both efficiently remove the important greenhouse gas CO2 and convert it to chemical products of high value. However, in addition to the configuration of electrochemical cells, electrocatalysts are main factors affecting key performances in electrochemical CO2 reduction reactions. Recently, studies have been conducted to investigate the roles of metal-based electrocatalysts and improve their performances through alloying, oxidization, and microstructural modulations. This review comprehensively discusses and analyzes the developments made in such metal-based electrocatalyst studies and presents the advancements of important metals for use in electrochemical CO2 reduction processes. The relationships between the electrodes' microstructure, chemistry, and efficiency in CO2 conversion are also compared and discussed.

中文翻译:

CO2高效电化学转化关键金属催化剂研究进展

电化学还原过程是有效去除重要的温室气体CO 2并将其转化为高价值化学产品的最有前景的方法之一。然而,除了电化学电池的配置,电催化剂是影响电化学CO 2还原反应关键性能的主要因素。最近,已经进行了研究以研究金属基电催化剂的作用,并通过合金化、氧化和微观结构调节来提高其性能。本综述全面讨论和分析了此类金属基电催化剂研究的进展,并介绍了用于电化学 CO 2的重要金属的进展还原过程。还比较和讨论了电极的微观结构、化学性质和 CO 2转化效率之间的关系。
更新日期:2022-06-27
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