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Atomically Dispersed Janus Nickel Sites on Red Phosphorus for Photocatalytic Overall Water Splitting
Angewandte Chemie International Edition ( IF 16.6 ) Pub Date : 2022-05-06 , DOI: 10.1002/anie.202204711
Menglong Wang, Shuai Xu, Zhaohui Zhou, Chung-Li Dong, Xu Guo, Jeng-Lung Chen, Yu-Cheng Huang, Shaohua Shen, Yubin Chen, Liejin Guo, Clemens Burda

A reactive-group guided approach is taken to synthesize atomically dispersed Ni catalysts on red phosphorus. The advanced system consists of Janus single-atom Ni sites: P−Ni for water reduction and P−O−Ni for water oxidation, leading to the efficient separation of electron-hole pairs and overall improved photocatalytic water splitting activity.

中文翻译:

红磷上原子分散的 Janus 镍位点用于光催化全水分解

采用反应基团引导的方法在红磷上合成原子分散的镍催化剂。先进的系统由 Janus 单原子 Ni 位点组成:用于水还原的 P-Ni 和用于水氧化的 P-O-Ni,导致电子-空穴对的有效分离和整体提高的光催化水分解活性。
更新日期:2022-05-06
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