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A hybrid model to improve WRF-Chem performance for crop burning emissions of PM2.5 and secondary aerosols in North India
Urban Climate ( IF 6.4 ) Pub Date : 2022-01-11 , DOI: 10.1016/j.uclim.2022.101084
Pavan K. Nagar 1 , Mukesh Sharma 1
Affiliation  

In north India (about 30,000 km2 area), October–November months witness crop residue burning (CRB). This study aims to assess the impact of CRB emissions on PM2.5 and secondary aerosol (SA) at distances far from the sources. Chemical transport model, WRF-Chem (with chemical mechanisms, RADM2 and MADE/SORGAM), was applied to a domain of 840 × 840 km2 (centered around Delhi) with inputs of emissions of anthropogenic sources of EDGAR-HTAP and fire inventory from the National Centre for Atmospheric Research, USA. In parallel, measurements of PM2.5 and its constituents, CO, and NO2 were undertaken in Delhi and Kanpur. The model underestimated PM2.5 and showed poor predictions (r < 0.15) with insignificant formation of secondary organic aerosol (SOA) (< 1% in PM2.5). To improve the model, a linear regression-based hybrid model (HM) was developed that utilized the mechanistic processes of WRF-Chem and observed levels of PM2.5, CO and NO2. The HM performed adequately at multiple sites in Delhi (r = 0.19–0.47) and Kanpur (r = 0.38–0.43). The contribution of CRB to PM2.5 was at 31 ± 16% (in 232 ± 36 μg/m3) in Delhi and 21 ± 15% (in 233 ± 38 μg/m3) in Kanpur. The contribution of SOA in CRB-contributed PM2.5 was 18 ± 9% (Delhi) and 29 ± 21% (Kanpur).



中文翻译:

一种混合模型,用于改善印度北部 PM2.5 和二次气溶胶的作物燃烧排放的 WRF-Chem 性能

在印度北部(约 30,000 km 2区域),10 月至 11 月的几个月见证了作物残茬燃烧 (CRB)。本研究旨在评估 CRB 排放对远离源头的PM 2.5和二次气溶胶 (SA) 的影响。化学传输模型 WRF-Chem(具有化学机制,RADM2 和 MADE/SORGAM)应用于 840 × 840 km 2(以德里为中心)的域,输入 EDGAR-HTAP 的人为排放源和火灾清单美国国家大气研究中心。同时,在德里和坎普尔对 PM 2.5及其成分、CO 和 NO 2进行了测量。该模型低估了 PM 2.5并显示出较差的预测 (r  < 0.15),二次有机气溶胶 (SOA) 的形成微不足道(在 PM 2.5 中< 1% )。为了改进模型,开发了一个基于线性回归的混合模型 (HM),该模型利用 WRF-Chem 的机械过程并观察到 ​​PM 2.5、CO 和 NO 2 的水平。HM 在德里 ( r  = 0.19–0.47) 和坎普尔 ( r  = 0.38–0.43) 的多个地点表现良好。CRB 对 PM 2.5的贡献在德里为 31 ± 16%(在 232 ± 36 μg/m 3 中),在坎普尔为21 ± 15%(在 233 ± 38 μg/m 3 中)。SOA 在 CRB 贡献的 PM 2.5中的贡献为 18 ± 9%(德里)和 29 ± 21%(坎普尔)。

更新日期:2022-01-11
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