Controlled Asymmetric Charge Distribution of Active Centers in Conjugated Polymers for Oxygen Reduction,Angewandte Chemie International Edition

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Controlled Asymmetric Charge Distribution of Active Centers in Conjugated Polymers for Oxygen Reduction
Angewandte Chemie International Edition ( IF 16.6 ) Pub Date : 2021-09-29 , DOI: 10.1002/anie.202109057
Daohao Li _{1,

2} , Binbin Wang _{1,

2} , Xiaojing Long _{1,

2} , Wenjia Xu ₁ , Yanzhi Xia ₁ , Dongjiang Yang _{1,

3} , Xiangdong Yao ₄

Affiliation

Metal-free conjugated polymer (CP) catalysts were developed with different degrees of asymmetry. The polymer catalyst with both asymmetric backbone and sidechain configuration provides larger dipole moment, regulated charge distribution, and higher ORR catalytic activity.