当前位置: X-MOL 学术Phys. Rev. Materials › 论文详情
Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)
Alloying-induced enhancement of thermopower in the Dirac-semimetal systemCd3−xZnxAs2
Physical Review Materials ( IF 3.4 ) Pub Date : 2021-09-07 , DOI: 10.1103/physrevmaterials.5.094201
J. Fujioka 1 , M. Kriener 2 , D. Hashizume 2 , Y. Yamasaki 3 , Y. Taguchi 2 , Y. Tokura 2, 4, 5
Affiliation  

Cd3As2 is one of the prototypical topological Dirac semimetals. Here, we manipulate the band inversion responsible for the emergence of Dirac nodes by alloying Cd3As2 with topologically trivial Zn3As2. The carrier density monotonically decreases and the resistivity is enhanced as x is increased. For larger x, the thermoelectric figure of merit exhibits comparably large values exceeding 0.3 at room temperature, due to the combined effects of a strong enhancement of the thermopower, an only moderate increase in the resistivity, and a suppression of the thermal conductivity. Complementary quantum-oscillation data and optical-conductivity measurements allow us to infer that the Dirac nodes are gapped out, and a band structure with a partly flat dispersion likely emerges in the higher-x region in Cd3xZnxAs2.

中文翻译:

Dirac-半金属系统Cd3−xZnxAs2 中合金化诱导的热电势增强

光盘3作为2是典型的拓扑狄拉克半金属之一。在这里,我们通过合金化来操纵导致狄拉克节点出现的能带反转光盘3作为2 与拓扑无关 3作为2. 载流子密度单调降低,电阻率提高为X增加。对于更大的X,由于热电势的强烈增强、电阻率仅适度增加和热导率的抑制的综合影响,热电品质因数在室温下表现出相对较大的值,超过 0.3。互补的量子振荡数据和光导率测量使我们能够推断狄拉克节点是有间隙的,并且在更高的区域可能会出现具有部分平坦色散的带结构。X 地区在 光盘3-XX作为2.
更新日期:2021-09-07
down
wechat
bug