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Self-heating-induced electrical and optical switching in high quality VO2 films controlled with current pulses
Journal of Materials Science: Materials in Electronics ( IF 2.8 ) Pub Date : 2021-09-06 , DOI: 10.1007/s10854-021-06895-2
Ozan Gunes 1 , Cyril Koughia 1 , Chunzi Zhang 1 , Safa O. Kasap 1 , George Belev 2 , Shi-Jie Wen 3 , Qiaoqin Yang 4
Affiliation  

Self-heating (SH)-induced electrical and optical switching in high quality VO2 films grown by magnetron sputtering on a c-cut sapphire substrate has been investigated under various applied constant current pulses (ID). The effect of SH on the behavior of electrical conductivity (σ), optical transmittance (\(\tilde{T })\), and film temperature (T) examined by applying a constant current pulse of various magnitudes with a pulse duration of five seconds (Δt = 5 s) in VO2 films which were pre-heated to and stabilized at 57 °C, at the brink of insulator-to-metal transition (IMT). The SH effect that arose from the application of constant ID pulses led to a significant increase in T and substantial changes in σ and \(\tilde{T }\). Observations showed that, depending on the magnitude of ID, the σ and \(\tilde{T }\) demonstrate strikingly different temporal behavior not only during the SH-induced IMT but also after the removal of ID. The observed phenomena could be explained using a simple model based on percolation theory previously proposed for the present system. The outcome of the model is confirmed by the results of the structural IMT obtained by Raman micromapping.



中文翻译:

电流脉冲控制的高质量 VO2 薄膜中的自热感应电和光开关

自加热(SH)在高品质诱导电气和光学开关VO 2层通过磁控溅射在c切割蓝宝石衬底上生长的薄膜各种施加恒定电流脉冲(下已经研究d)。SH 对电导率 ( σ )、透光率 ( \(\tilde{T})\)和薄膜温度 ( T ) 行为的影响,通过施加不同幅度的恒定电流脉冲,脉冲持续时间为 5秒 (Δ t  = 5 s) 在 VO 2薄膜中,该薄膜预热至并稳定在 57 °C,处于绝缘体到金属转变 (IMT) 的边缘。应用常数引起的 SH 效应I D脉冲导致T的显着增加以及σ\(\tilde{T }\)的显着变化。观察表明,根据I D的大小,σ\(\tilde{T }\)不仅在 SH 诱导的 IMT 期间而且在去除I D之后都表现出显着不同的时间行为。可以使用基于先前为本系统提出的渗透理论的简单模型来解释观察到的现象。通过拉曼显微成像获得的结构 IMT 结果证实了模型的结果。

更新日期:2021-09-06
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