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Cross-dehydrogenative coupling: a sustainable reaction for C–C bond formations
Green Chemistry ( IF 9.8 ) Pub Date : 2021-07-23 , DOI: 10.1039/d1gc01871j
Tian Tian 1 , Zhiping Li 1 , Chao-Jun Li 2
Affiliation  

We are entering an era that emphasizes greenness and sustainability. Based on such a philosophy, it is critical to uncover novel and original sustainable reaction modes for future green chemical syntheses. The cross-dehydrogenative coupling (CDC) reaction has thus been widely developed as one of the most sustainable and efficient synthesis strategies for constructing C–C bonds. This review summarizes the development of this field over the past 20 years, with a discussion on future trends and directions: from the original reaction model at the beginning and its development in the first decade, to extensive research in the second decade. The latest development sees the emergence of alternative forms of energy inputs (photoredox, mechano, microwave, electrochemical, continuous-flow and solar quantum dots) to facilitate CDC reactions, gradually replacing the classical form of thermal energy, which will inspire broader applications and innovations in the future.

中文翻译:

交叉脱氢偶联:C-C 键形成的可持续反应

我们正在进入一个强调绿色和可持续性的时代。基于这样的理念,为未来的绿色化学合成发现新颖和原始的可持续反应模式至关重要。因此,交叉脱氢偶联(CDC)反应已被广泛发展为构建 C-C 键的最可持续和最有效的合成策略之一。这篇综述总结了该领域过去20年的发展,并讨论了未来的趋势和方向:从最初的原始反应模型和第一个十年的发展,到第二个十年的广泛研究。最新的发展看到了替代形式的能量输入(光氧化还原、机械、微波、电化学、连续流和太阳能量子点)的出现,以促进 CDC 反应,
更新日期:2021-08-27
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