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Development and testing of a Delayed Gamma-ray Spectroscopy instrument utilizing Cf-252 neutrons evaluated for nuclear safeguards applications
Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment ( IF 1.4 ) Pub Date : 2021-07-26 , DOI: 10.1016/j.nima.2021.165685
Douglas Chase Rodriguez 1 , Kamel Abbas 2 , Mitsuo Koizumi 1 , Stefan Nonneman 2 , Fabiana Rossi 1 , Tohn Takahashi 1
Affiliation  

The Japan Atomic Energy Agency (JAEA) is collaborating with the European Commission Joint Research Centre (EC/JRC) to develop delayed gamma-ray spectroscopy (DGS). Toward this, the JAEA Integrated Support Center for Nuclear Nonproliferation and Nuclear Security (ISCN) designed the Delayed Gamma-ray Test Spectrometer (DGTS) that uses a 252Cf source (DGTS-C). This instrument is used to refine the design for a compact, induced-fission safeguards technique to supplement current nuclear material accountancy in reprocessing facilities. Experiments were performed at PERLA laboratory of the EC/JRC Ispra, Italy site to evaluate the neutron-irradiation and associated instrumentation capabilities to obtain delayed gamma-ray spectral signatures of assayed nuclear material. Neutron count-rate measurements were performed using a 3He detector and confirmed with MCNP6 models that showed a fluence of ∼87.1×104 n cm−2 nsrc1. Short time-pattern interrogations of various 235U and 239Pu samples resulted in quantifiable delayed gamma-ray peaks from fission products. The peak intensities and spectral signatures resulted in fissile nuclide distinction and linear mass-correlation results. Consequently, we confirm the practicality of this JAEA/ISCN instrument design for DGS interrogation safeguards capabilities.



中文翻译:

利用 Cf-252 中子开发和测试用于核保障应用的延迟伽马射线光谱仪

日本原子能厅 (JAEA) 正在与欧盟委员会联合研究中心 (EC/JRC) 合作开发延迟伽马射线光谱 (DGS)。为此,JAEA 核不扩散和核安全综合支持中心 (ISCN) 设计了延迟伽马射线测试光谱仪 (DGTS),它使用252Cf 源 (DGTS-C)。该仪器用于改进紧凑型诱导裂变保障技术的设计,以补充后处理设施中当前的核材料衡算。在 EC/JRC Ispra 意大利站点的 PERLA 实验室进行了实验,以评估中子辐照和相关仪器的能力,以获得化验核材料的延迟伽马射线光谱特征。中子计数率测量是使用3 He 探测器进行的,并用 MCNP6 模型进行了确认,该模型显示了 ∼87.1×10-4n cm -2 nrC-1. 对各种235 U 和239 Pu 样品的短时间模式询问导致裂变产物产生可量化的延迟伽马射线峰。峰值强度和光谱特征导致裂变核素区分和线性质量相关结果。因此,我们确认了这种用于 DGS 审讯保障能力的 JAEA/ISCN 仪器设计的实用性。

更新日期:2021-08-12
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