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Elastoplasticity Mediates Dynamical Heterogeneity Below the Mode Coupling Temperature
Physical Review Letters ( IF 8.6 ) Pub Date : 2021-07-22 , DOI: 10.1103/physrevlett.127.048002
Rahul N Chacko 1, 2 , François P Landes 3 , Giulio Biroli 4 , Olivier Dauchot 5 , Andrea J Liu 1 , David R Reichman 6
Affiliation  

As liquids approach the glass transition temperature, dynamical heterogeneity emerges as a crucial universal feature of their behavior. Dynamic facilitation, where local motion triggers further motion nearby, plays a major role in this phenomenon. Here we show that long-ranged, elastically mediated facilitation appears below the mode coupling temperature, adding to the short-range component present at all temperatures. Our results suggest deep connections between the supercooled liquid and glass states, and pave the way for a deeper understanding of dynamical heterogeneity in glassy systems.

中文翻译:

弹塑性在模式耦合温度以下介导动态非均匀性

随着液体接近玻璃化转变温度,动态异质性成为其行为的关键普遍特征。动态促进,其中局部运动触发附近的进一步运动,在这种现象中起着重要作用。在这里,我们表明长程、弹性介导的易化出现在模式耦合温度以下,增加了在所有温度下都存在的短程分量。我们的结果表明过冷液体和玻璃状态之间存在深层联系,并为更深入地了解玻璃系统中的动态异质性铺平了道路。
更新日期:2021-07-22
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