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Gap plasmon modes resolved by ultraflat nanogap and linear polarization in terrace-stepped hexagonal boron nitride spacer sandwiched by Ag nanowire and metal substrates
Current Applied Physics ( IF 2.4 ) Pub Date : 2021-07-17 , DOI: 10.1016/j.cap.2021.07.008
Kyoung-Ho Kim 1 , Jubok Lee 2 , Evan S.H. Kang 1 , Dong-Hyun Kim 1 , Hyun Seok Lee 1
Affiliation  

We investigate the nanogap and polarization-resolved excitation of gap plasmon modes using terrace-stepped hexagonal boron nitride (hBN) sandwiched between Ag nanowires and Au substrates for a metal–insulator–metal gap structure. The gap plasmon modes in the proposed hybrid structure are dominantly excited by a P-polarized incident light, which is supported by full-wave numerical simulations. Plasmon mode evolution for various hBN spacer thicknesses ranging from 5 to 90 nm shows that optical signals acquired via unpolarized dark-field mapping spectroscopy are primarily due to the optical scattering of the P-polarized incident light. Moreover, this plasmonic mode changes significantly from gap plasmon mode to Fabry–Perot-type resonance in a hBN thickness of 50–90 nm. Our analysis reveals that the proposed hybrid structure based on Ag nanowires and stepped hBN provides a well-defined gap thickness and is a robust platform for analyzing gap plasmon modes.



中文翻译:

由银纳米线和金属基板夹在梯田阶梯形六方氮化硼间隔物中的超平坦纳米间隙和线性极化解析间隙等离子体模式

我们使用夹在 Ag 纳米线和 Au 衬底之间的阶梯阶梯式六方氮化硼 (hBN) 来研究间隙等离子体模式的纳米间隙和极化分辨激发,以形成金属-绝缘体-金属间隙结构。所提出的混合结构中的间隙等离子体模式主要由 P 偏振入射光激发,这得到了全波数值模拟的支持。从 5 到 90 nm 的各种 hBN 间隔层厚度的等离子体模式演化表明,通过非偏振暗场映射光谱获得的光信号主要是由于 P 偏振入射光的光学散射。此外,这种等离子体模式在 hBN 厚度为 50-90 nm 时从间隙等离子体模式显着改变为法布里-珀罗型共振。

更新日期:2021-07-22
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