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Drastic reduction of theR-Fe exchange in interstitially modified(Nd,Ho)2Fe14Bcompounds probed by megagauss magnetic fields
Physical Review Materials ( IF 3.4 ) Pub Date : 2021-07-09 , DOI: 10.1103/physrevmaterials.5.074404
N. V. Kostyuchenko 1 , I. S. Tereshina 2 , E. A. Tereshina-Chitrova 3, 4 , L. A. Ivanov 2 , M. Paukov 4, 5 , D. I. Gorbunov 6 , A. V. Andreev 3 , M. Doerr 7 , G. A. Politova 8, 9 , A. K. Zvezdin 10, 11 , S. V. Veselova 2 , A. P. Pyatakov 2 , A. Miyata 12 , O. Drachenko 12 , O. Portugall 12
Affiliation  

In this paper, the full magnetization process demonstrated by the series of ferrimagnetic intermetallic compounds (Nd,Ho)2Fe14B and Ho2Fe14B and their hydrides with the maximum possible hydrogen content (for the given crystal structure type) is studied theoretically and experimentally using megagauss magnetic fields. We observe field-induced phase transitions from the initial ferrimagnetic to the forced-ferromagnetic state in magnetic fields up to 130 T and describe the magnetization process analytically. We find a drastic decrease of the critical transition fields in the hydrogenated compounds. This is due to extremely strong, nearly twofold reduction of the R-Fe intersublattice exchange interaction because of the combined substitution and hydrogenation effects. A comparative analysis of the magnetization behavior for the system Ho2Fe17H is also performed.

中文翻译:

超高斯磁场探测的间隙改性(Nd,Ho)2Fe14B化合物中R-Fe交换的急剧减少

在本文中,由一系列亚铁磁性金属间化合物证明的全磁化过程 (,)214214并且使用兆高斯磁场从理论上和实验上研究了具有最大可能氢含量(对于给定的晶体结构类型)的氢化物。我们在高达 130 T 的磁场中观察到从初始亚铁磁态到强制铁磁态的场致相变,并分析地描述了磁化过程。我们发现氢化化合物中的临界跃迁场急剧下降。这是由于极强的,几乎两倍的减少电阻-Fe 晶间交换相互作用,因为结合的取代和氢化效应。系统磁化行为的比较分析217-H 也进行。
更新日期:2021-07-09
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