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CO2 separation by rotating liquid sheet contactor: A novel procedure to improve mass transfer characterization
Chemical Engineering Research and Design ( IF 3.9 ) Pub Date : 2021-06-15 , DOI: 10.1016/j.cherd.2021.06.008
Morteza Mehdipour , Abbas Elhambakhsh , Peyman Keshavarz , Mohammad Reza Rahimpour , Yasha Hasanzadeh

In this work, the rotating liquid sheet (RLS) contactor was used as a new contactor device for the separation of CO2 content from CO2/N2 gas mixtures by pure water, MDEA and DEA solutions. To do so, an RLS module with a helical slot in the wall of central tube was designed to provide a single continues helical liquid sheet with high levels of the liquid–gas contact area. Subsequently, the influence of various operating parameters including gas flow rate, CO2 inlet concentration and solvent concentration was investigated. The obtained results clearly revealed that separation efficiency could reach higher than 95% by DEA solution. Also, experimental observations proved that with increasing the gas flow rate and CO2 inlet concentration, the absorption flux increases while the separation efficiency reduces. In addition, the CO2 removal process can be improved by increment solvent concentration. Further, as a unique advantage, tube rotation intensified mass transfer from the gas stream into the liquid absorbents.



中文翻译:

通过旋转液片接触器分离CO 2:一种改进传质表征的新方法

在这项工作中,旋转液片 (RLS) 接触器被用作一种新的接触器装置,用于通过纯水、MDEA 和 DEA 溶液从 CO 2 /N 2气体混合物中分离 CO 2含量。为此,设计了一个在中心管壁上带有螺旋槽的 RLS 模块,以提供具有高液气接触面积的单个连续螺旋液体层。随后,研究了包括气体流速、CO 2入口浓度和溶剂浓度在内的各种操作参数的影响。所得结果清楚地表明,DEA 溶液的分离效率可达到 95% 以上。此外,实验观察证明,随着气体流速和 CO 2入口浓度,吸收通量增加,而分离效率降低。此外,可以通过增加溶剂浓度来改进CO 2去除过程。此外,作为一个独特的优势,管子旋转加强了从气流到液体吸收剂的传质。

更新日期:2021-06-18
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