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Simple and efficient method for producing high radionuclidic purity 111In using enriched 112Cd target
Applied Radiation and Isotopes ( IF 1.6 ) Pub Date : 2021-06-13 , DOI: 10.1016/j.apradiso.2021.109828
Jing Gao 1 , Zhonghui Liao 1 , Weihao Liu 1 , Yingjiang Hu 1 , Huan Ma 1 , Lingting Xia 1 , Feize Li 1 , Tu Lan 1 , Yuanyou Yang 1 , Jijun Yang 1 , Jiali Liao 1 , Ning Liu 1
Affiliation  

In this work, a simple and efficient method for producing high radionuclidic purity 111In from an enriched 112Cd target was developed. The enriched 112Cd metal target formed by cyanide-free electroplating was bombarded with protons of 21 MeV in a CS-30 cyclotron. Then, we explored a purification scheme using CL-P204 cation exchange resin wherein 98% of the 111In in the bombarded target could be extracted in less than 1 h. The purified 111In in the form of [111In]In-chloride had a high radionuclidic purity (99.9%) and a low impurity concentration (<1.2 ppm). The yield of 111In via the reaction of 112Cd (p, 2n) 111In was measured to be 222 ± 5 MBq/μA∙h. In addition, a chemical procedure for collecting the unreacted 112Cd at a recovery rate of 96.6% was explored.



中文翻译:

使用富集 112Cd 靶材生产高放射性核素纯度 111In 的简单有效方法

在这项工作中,开发了一种从富集的112 Cd 靶中生产高放射性核素纯度111 In的简单有效的方法。通过无氰电镀形成的富集112 Cd 金属靶在 CS-30 回旋加速器中用 21 MeV 的质子轰击。然后,我们探索了使用 CL-P204 阳离子交换树脂的纯化方案,其中可以在不到 1 小时的时间内提取出轰击目标中98% 的111 In。[ 111 In] In-氯化物形式的纯化111 In具有高放射性核素纯度(99.9%)和低杂质浓度(<1.2 ppm)。112 Cd (p, 2n) 111反应生成111 InIn 测量值为 222 ± 5 MBq/μA∙h。此外,还探索了一种以 96.6% 的回收率收集未反应的112 Cd的化学程序。

更新日期:2021-06-21
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