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Theoretical studies on the cascade decay processes of 1s-core-hole state of Ar ion
Journal of Electron Spectroscopy and Related Phenomena ( IF 1.9 ) Pub Date : 2021-05-15 , DOI: 10.1016/j.elspec.2021.147083
X.L. Wang , B.X. Liu , G.H. Zhang , P.Y. Wang , L.W. Liu , X.Y. Li

The cascade decay processes from the 1s-core-hole state of Ar ion have been studied theoretically via straightforward construction of de-excitation trees and high-accuracy level-to-level calculations using the flexible atomic code (FAC). The final charge state distribution (FCSD), contributions of different cascade routes to the FCSD, and the main production pathways of each Ari+ ion which are never discussed before are analyzed carefully. It is found that the de-excitation processes is very complex and Auger decay is the predominant channel, the most probable final charge state is 4, while Ar+ to Ar6+ ions can be produced in the 5-step Auger cascade decay processes for Ar+1s−1 hole state. Ar+ is mainly derived from KM23 channel, Ar2+ is associated mainly with KL23 channel, when Ar3+, Ar4+, Ar5+ and Ar6+ions are mainly coming from KL23M23, KL23L23, KL1L23 and KL1L1 channels, respectively. Present studies would be helpful for further researches on the cascade decay processes of deep inner-shell hole states, and for the interaction between x-ray free-electron lasers and matter.



中文翻译:

Ar离子1s核孔态级联衰变过程的理论研究

从理论上讲,通过简单地构建消磁树并使用柔性原子代码(FAC)进行高精度的逐级计算,研究了Ar离子从1s核孔态的级联衰减过程。仔细分析了最终电荷状态分布(FCSD),不同级联路径对FCSD的贡献以及每个Ar i +离子的主要生产途径,这些都是以前从未讨论过的。发现去激励过程非常复杂,俄歇衰变是主要的通道,最可能的最终电荷态是4,而在5步俄歇级联衰变过程中,可以产生Ar +至Ar 6+离子。 Ar + 1s -1空穴状态。氩+当Ar 3+,Ar 4+,Ar 5+和Ar 6+离子主要来自KL 23 M 23,KL 23 L 23时,Ar 2+主要来自KM 23通道,而Ar 2+主要与KL 23通道相关。 KL 1 L 23和KL 1 L 1通道。目前的研究将有助于进一步研究深壳内孔态的级联衰变过程,以及有助于X射线自由电子激光器与物质之间的相互作用。

更新日期:2021-05-22
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