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Numerical modelling of CO2 migration in heterogeneous sediments and leakage scenario for STEMM-CCS field experiments
International Journal of Greenhouse Gas Control ( IF 3.9 ) Pub Date : 2021-04-29 , DOI: 10.1016/j.ijggc.2021.103339
Umer Saleem , Marius Dewar , Tariq Nawaz Chaudhary , Mehroz Sana , Anna Lichtschlag , Guttorm Alendal , Baixin Chen

The dynamics and plume development of injected CO2 dispersion and dissolution through sediments into water column, at the STEMM-CCS field experiment conducted in Goldeneye, are simulated and predicted by a newly developed two-phase flow model based on Navier-Stokes-Darcy equations. In the experiment, CO2 gas was released into shallow marine sediment 3.0 m below the seafloor at 120 m water depth in the North Sea.

The pre-experimental survey data of porosity, grain size distributions, and brine concentration are used to reconstruct the model sediments. The gas CO2 is then injected into the sediments at a rate of 5.7 kg/day to 143 kg/day. The model is validated by diagnostic simulations to compare with field observation data of CO2 eruption time, changes in pH in sediments, and the gas leakage rates. Then the dynamics of the CO2 plume development in the sediments are investigated by model simulations, including the leakage pathways, the fluids interactions among CO2/brine/sediments, and CO2 dissolution, in order to comprehend the mechanisms of CO2 leakage through sediments. It is shown from model simulations that the CO2 plume develops horizontally in the sediments at a rate of 0.375 m/day, CO2 dissolution in the sediments is at an overall average rate of 0.03 g/sec with some peaks of 0.45 g/sec, 0.15 g/sec, and 0.3 g/sec, respectively, following the increase in injection rates, when some fresh brine provided. These, therefore, lead to a ratio of 0.90~0.93 of CO2 leakage rate to injection rate.



中文翻译:

STEMM-CCS现场实验中非均质沉积物中CO 2迁移的数值模拟和渗漏情景

通过在新开发的基于Navier-Stokes-Darcy方程的两相流模型中进行模拟和预测,在Goldeneye进行的STEMM-CCS现场实验中,模拟并预测了注入的CO 2通过沉积物分散和溶解到水柱中的动力学和羽状流发展。。在实验中,CO 2气体被释放到北海水深120 m处海床以下3.0 m的浅海沉积物中。

实验前的孔隙率,粒度分布和盐水浓度调查数据可用于重建模型沉积物。然后将气体CO 2以5.7 kg /天至143 kg /天的速度注入沉积物中。该模型已通过诊断模拟验证,可以与CO 2喷发时间,沉积物的pH值变化以及漏气率的现场观测数据进行比较。然后通过模型模拟研究了沉积物中CO 2羽状流发育的动力学,包括泄漏途径,CO 2 /盐水/沉积物之间的流体相互作用以及CO 2溶解,以了解CO 2的机理。通过沉积物泄漏。从模型模拟中可以看出,CO 2羽以0.375 m / day的速率在沉积物中水平发展,CO 2在沉积物中的溶解以0.03 g / sec的总体平均速率分布,有些峰值为0.45 g / sec当注入一些新鲜盐水时,随着注入速率的增加,分别为0.15 g / sec和0.3 g / sec。因此,这些导致CO 2泄漏率与注入率之比为0.90〜0.93 。

更新日期:2021-04-30
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