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Polyelectrolyte Complex Coacervates: Recent Developments and New Frontiers
Annual Review of Condensed Matter Physics ( IF 22.6 ) Pub Date : 2021-03-10 , DOI: 10.1146/annurev-conmatphys-042020-113457
Artem M. Rumyantsev 1 , Nicholas E. Jackson 1, 2 , Juan J. de Pablo 1, 2
Affiliation  

Polyelectrolyte complex coacervates represent a wide class of materials with applications ranging from coatings and adhesives to pharmaceutical technologies. They also underpin multiple biological processes, which are only now beginning to be deciphered. The means by which molecular-scale architecture propagates into macroscopic structure, thermodynamics, and dynamics in complex coacervates is of central concern in physics, chemistry, biology, and materials science. How does polyion charge sequence dictate thermodynamic behavior? How does one tailor rheology or interfacial tension using macromolecular architecture? What emergent functionality from polymer complex coacervates has biological consequences? Recent developments in coacervate science shed light on many of these issues and raise exciting new challenges for the close integration of theory, simulations, and experiment.

中文翻译:


聚电解质复合物凝聚层:最新发展和新领域

聚电解质复合凝聚层代表了各种各样的材料,其应用范围从涂料和粘合剂到制药技术。它们还支持多种生物学过程,而这些生物学过程才刚刚开始被破译。在复杂凝聚层中,分子尺度结构传播到宏观结构,热力学和动力学的方法是物理,化学,生物学和材料科学的中心问题。聚离子的电荷顺序如何决定热力学行为?如何利用大分子结构调整流变学或界面张力?聚合物复合物凝聚层中出现的哪些新功能会产生生物学后果?凝聚科学的最新发展为许多这些问题提供了启示,并为理论的紧密结合提出了令人振奋的新挑战,

更新日期:2021-03-10
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