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Thermodynamics of Fluorite-Structured Oxides Relevant to Nuclear Energy: A Review
ACS Earth and Space Chemistry ( IF 3.4 ) Pub Date : 2021-02-09 , DOI: 10.1021/acsearthspacechem.0c00199
Anna Shelyug 1 , Alexandra Navrotsky 2
Affiliation  

Fluorite structured materials have shown their applicability in various fields both on and off Earth. In particular, these oxides find extensive application in nuclear energy and the use of actinides in space and planetary settings, thermal and environmental barrier coatings, aerospace applications, catalysts, fuel cells, and batteries. Research done on thermodynamic data collection should be structured to facilitate its use in predictive calculations. In this review, we bring together several decades of experimental thermodynamic analysis of fluorite-based oxides with an emphasis on their relevance to all stages of the nuclear fuel cycle. This review is relatively short in the interest of offering an accessible perspective, especially for scientists early in their careers in nuclear science.

中文翻译:

与核能有关的萤石结构氧化物的热力学:综述

萤石结构材料已显示出其在地球上和地球外各个领域的适用性。特别是,这些氧化物在核能中广泛应用,并在空间和行星环境,热和环境屏障涂层,航空航天应用,催化剂,燃料电池和电池中使用act系元素。应该对热力学数据收集进行研究,以促进其在预测计算中的使用。在这篇综述中,我们将对基于萤石的氧化物进行数十年的实验热力学分析,重点放在它们与核燃料循环所有阶段的相关性上。这篇评论相对较短,目的是提供一种可访问的观点,特别是对于在核科学事业早期的科学家而言。
更新日期:2021-03-18
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