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Heterogeneous Water Oxidation Catalysts for Molecular Anodes and Photoanodes
Solar RRL ( IF 7.9 ) Pub Date : 2021-01-05 , DOI: 10.1002/solr.202000565
Matthew V. Sheridan 1 , Benjamin D. Sherman 2 , Yi Xie 3 , Ying Wang 3
Affiliation  

Water oxidation is a critical half reaction in alternative energy and essential to producing solar fuels from light-driven water splitting. Molecular complexes, especially those based on ruthenium, represent a promising class of catalysts for use in these systems. Studies of ruthenium complexes in homogeneous solutions represent an overwhelming majority of the literature on molecular catalysts thus far. Nonetheless, the development of devices for light-driven water splitting necessitates the translation of catalysts to surfaces, namely, semiconductor metal-oxide surfaces. Progress in this equally important area of heterogeneous molecular water oxidation and mechanistic studies at surfaces is reviewed herein.

中文翻译:

用于分子阳极和光阳极的多相水氧化催化剂

水氧化是替代能源中的关键半反应,对于通过光驱动水分解生产太阳能燃料至关重要。分子复合物,尤其是那些基于钌的复合物,代表了一类有前途的催化剂,可用于这些系统。迄今为止,在均相溶液中对钌配合物的研究占绝大多数关于分子催化剂的文献。尽管如此,光驱动水分解装置的开发需要将催化剂转化为表面,即半导体金属氧化物表面。本文综述了异质分子水氧化和表面机理研究这一同等重要领域的进展。
更新日期:2021-01-05
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