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Utilization of Trapped Optical Modes for White Perovskite Light-Emitting Diodes with Efficiency over 12%
Joule ( IF 39.8 ) Pub Date : 2021-01-04 , DOI: 10.1016/j.joule.2020.12.008
Ziming Chen , Zhenchao Li , Zhen Chen , Ruoxi Xia , Guangruixing Zou , Linghao Chu , Shi-Jian Su , Junbiao Peng , Hin-Lap Yip , Yong Cao

The inferior light extraction efficiency (LEE), which is generally less than 20%, based on optical modeling, and the difficulty in achieving white emission are the two main challenges in the metal-halide-perovskite light-emitting diode (PeLED) field. Herein, we report a simple and efficient approach to construct high-performance white PeLEDs with much-enhanced LEE by coupling a blue PeLED with a layer of red perovskite nanocrystal (PeNC) down-converter through a rationally designed multilayer semitransparent electrode (LiF/Al/Ag/LiF). The red PeNC layer allows the extraction of the trapped waveguide mode and surface plasmon polariton mode in a blue PeLED and converts them to red emission, resulting in over 50% LEE improvement. Simultaneously, the complementary emission spectrum of blue photons and down-converting red photons contributes to a white PeLED with a high external quantum efficiency and luminance of more than 12% and approximately 2,000 cd m−2, respectively, which represent state-of-the-art results in this field.



中文翻译:

捕获的光模用于白色钙钛矿发光二极管的效率超过12%

基于光学模型,劣质的光提取效率(LEE)通常低于20%,难以实现白色发射是金属卤化物-钙钛矿型发光二极管(PeLED)领域的两个主要挑战。在本文中,我们报告了一种简单有效的方法,通过合理设计的多层半透明电极(LiF / Al),将蓝色PeLED与红色钙钛矿纳米晶体(PeNC)下变频器层耦合,从而构建具有增强型LEE的高性能白色PeLED。 / Ag / LiF)。红色PeNC层允许提取蓝色PeLED中捕获的波导模式和表面等离子体激元极化模式,并将其转换为红色发射,从而使LEE改善了50%以上。同时,-2分别代表该领域的最新技术成果。

更新日期:2021-02-17
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