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Highly sensitive detection of H2O adsorbed on Si(111)7 × 7 and Si(100)2 × 1 surfaces by means of slow highly charged Xe ions
Surface Science ( IF 1.9 ) Pub Date : 2020-12-24 , DOI: 10.1016/j.susc.2020.121785
Satoshi Takahashi , Masahide Tona , Nobuyuki Nakamura , Chikashi Yamada , Makoto Sakurai , Shunsuke Ohtani

The proton yields from Si(111)7 × 7 and Si(100)2 × 1 reconstructed surfaces irradiated with slow (v<0.25vBohr) highly charged Xe ions are obtained. H2O molecules adsorbed over time on the surfaces at room temperature, under ultra-high vacuum can be detected as an increase of the proton yield. For the Si(100)2 × 1 surface, the proton yield with HCI-irradiation time is discussed based on temporal variation of the H2O coverage. The proton desorption efficiency with Xe50+ is more than about ten times and twice as compared with Xe29+ and Xe44+, respectively. For the Si(111)7 × 7 and Si(100)2 × 1 surfaces, the proton yield in each time increases with the charge states q to the power of 6 and 4, respectively, and is changed with time with the power laws held on.



中文翻译:

高度灵敏的检测 H2Ø 吸附在Si(111)7上 × 7和Si(100)2 × 1个表面,通过缓慢带电的Xe离子

质子从Si(111)7产生 × 7和Si(100)2 × 1慢速照射重建表面 v<0.25v玻尔 获得高电荷的Xe离子。 H2Ø随着质子产率的增加,在室温下,超高真空下,随着时间的推移吸附在表面上的分子可被检测到。对于Si(100)2 × 在图1的表面上,基于HCI的时间变化讨论了质子产率与HCI辐射时间的关系 H2Ø覆盖范围。质子解吸效率随e50+ 是十倍以上两倍 e29+e44+分别。对于Si(111)7 × 7和Si(100)2 × 1表面,每次质子产率随电荷态的增加而增加 q 分别乘以6和4的幂,并且在保持幂律不变的情况下随时间变化。

更新日期:2021-02-02
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