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Synthesis and interface modification of oxide solid-state electrolyte-based all-solid-state lithium-ion batteries: Advances and perspectives
Functional Materials Letters ( IF 1.3 ) Pub Date : 2020-12-19 , DOI: 10.1142/s1793604721300024
Linchun He 1 , Jin An Sam Oh 1, 2, 3 , Jun Jie Jason Chua 1 , Henghui Zhou 4
Affiliation  

All-solid-state Li-ion batteries (ASSLiBs) are considered as promising next-generation energy storage devices, and the one that is based on oxide ceramic solid-state electrolyte (SSE) has attracted much attention for its high safety and stability in ambient conduction compared with that of used sulfur and polymer SSEs. However, the undeformable nature of the ceramic SSEs brings new issues such as poor interface bonding, limited contact area and limited cathode utilization for the ASSLiBs. In addition, the interface reaction and resistance are also obstacles for ASSLiBs application. In this review, we focus on the synthesis and electrochemical properties, interface modification and failure mechanism of ASSLiBs. Finally, perspectives of future researches on the ceramic SSEs-based ASSLiBs are discussed.

中文翻译:

基于氧化物固态电解质的全固态锂离子电池的合成与界面改性:进展与展望

全固态锂离子电池(ASSLiBs)被认为是有前途的下一代储能装置,基于氧化物陶瓷固态电解质(SSE)的锂离子电池以其高安全性和稳定性而备受关注。与使用的硫和聚合物 SSE 的环境传导相比。然而,陶瓷 SSE 的不可变形特性带来了新的问题,例如界面结合不良、接触面积有限以及 ASSLiB 的阴极利用率有限。此外,界面反应和阻力也是ASSLiBs应用的障碍。在这篇综述中,我们重点关注 ASSLiBs 的合成和电化学性能、界面改性和失效机制。最后,讨论了基于陶瓷 SSE 的 ASSLiB 的未来研究前景。
更新日期:2020-12-19
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