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Spatial and temporal patterns of methane and its influencing factors in the Jiulong River estuary, southeastern China
Marine Chemistry ( IF 3 ) Pub Date : 2020-12-17 , DOI: 10.1016/j.marchem.2020.103909
Yuhong Li , Liyang Zhan , Liqi Chen , Jiexia Zhang , Man Wu , Jian Liu

Estuaries are important sources of methane (CH4) to the atmosphere. However, the lack of adequate field studies for understanding the sources/sinks of CH4 in estuaries hampers global atmospheric budgeting. Therefore, more studies are needed to bridge this gap and improve our understanding of CH4 dynamics. This study investigated the impacts of tides on CH4 emissions along a salinity gradient of the subtropical Jiulong River estuary (JRE) during spring, neap tides and over 24 h tidal cycles in 2017 and 2018. Spatially, the CH4 concentrations increased from the lower reaches to the upper reaches, with values varying widely from 58 to 1726 (393 ± 336) nmol/L, which correspond to saturations of 2513–59,371 (15,549 ± 11,341)%. The CH4 concentration was inversely and significantly correlated with salinity, indicating the dilution and sulfate inhibition effects of the adjacent saline water. Temporally, the highest CH4 concentrations and fluxes were detected in the spring tide period, which can enhance the resuspension of particles and CH4 from sediments, and were accompanied by high turbidity values. Elevated CH4 concentrations were found during low tide, and horizontal advection of low salinity water could be the driver of the increased CH4 concentrations during low tide. Due to the lack of agreement among current diffusive models, three different parameterizations were used to assess the water-air fluxes of CH4 in this study. The flux range was estimated to be 193–18,585 (2793 ± 3812) μmol/m2/d, which is well above that reported for most estuaries worldwide.



中文翻译:

东南九龙河口甲烷的时空分布特征及其影响因素

河口是大气中甲烷(CH 4)的重要来源。但是,缺乏足够的实地研究来了解河口CH 4的来源/汇,这妨碍了全球大气预算。因此,需要更多的研究来弥合这一差距并增进我们对CH 4动力学的理解。本研究调查潮汐的影响上CH 4个在2017年和2018年春季,小潮期间和24小时以上潮汐周期沿亚热带九龙江口(JRE)的盐度梯度排放空间,所述CH 4浓度从下游增加到上游,其值在58至1726(393±336)nmol / L之间变化很大,对应于2513–59,371(15,549±11,341)%的饱和度。CH 4浓度与盐度成反比且显着相关,表明相邻盐水的稀释和硫酸盐抑制作用。暂时,在春季潮汐时期检测到最高的CH 4浓度和通量,这可以增强颗粒和CH 4从沉积物中的重悬浮,并伴有较高的浊度值。在退潮期间发现CH 4浓度升高,低盐度水的水平对流可能是CH 4增加的驱动力在退潮时集中注意力。由于当前的扩散模型之间缺乏一致性,因此在本研究中使用了三种不同的参数化方法来评估CH 4的水-空气通量。通量范围估计为193–18,585(2793±3812)μmol/ m 2 / d,远高于全球大多数河口的报告范围。

更新日期:2020-12-17
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