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Graphene oxide-promoted Ti/PbO2 photoanode with photoelectric synergy effect for efficient photoelectrocatalytic degradation of reactive brilliant blue
Journal of Materials Science ( IF 4.5 ) Pub Date : 2020-11-30 , DOI: 10.1007/s10853-020-05604-4
Wenfeng Li , Huiru Ma-An , Yinghuan Fu , Chun Ma , Guowen Wang , Xiaoli Dong , Hongchao Ma

The development of semiconductor-based photoelectrocatalysts with superior activity is of great importance for water purification. Here, we fabricated graphene oxide (GO)-wrapped Ti/PbO2 photoanodes by combination of electrochemical deposition and electrophoretic deposition process. The as-obtained composite electrodes showed better performance for photoelectrocatalytic (PEC) degradation of reactive brilliant blue KN-R, as compared with that of Ti/PbO2 reference. Experimental results demonstrated that the efficient PEC performance of graphene oxide (GO)-wrapped Ti/PbO2 photoanodes could be ascribed to the low charge transfer resistance, large electrochemical active areas, and high separation efficiency of induced electrons/holes. Furthermore, a significant photoelectric synergy effect can be observed for the graphene oxide (GO)-wrapped Ti/PbO2 photoanodes during the photoelectrocatalytic process.

中文翻译:

具有光电协同效应的氧化石墨烯促进的 Ti/PbO2 光阳极用于高效光电催化降解活性艳蓝

开发具有优异活性的半导体基光电催化剂对于水净化具有重要意义。在这里,我们通过电化学沉积和电泳沉积工艺的结合制造了氧化石墨烯(GO)包裹的 Ti/PbO2 光阳极。与 Ti/PbO2 参比相比,所获得的复合电极对反应性艳蓝 KN-R 的光电催化(PEC)降解表现出更好的性能。实验结果表明,氧化石墨烯(GO)包裹的 Ti/PbO2 光阳极的高效 PEC 性能可归因于低电荷转移电阻、大电化学活性区域和高诱导电子/空穴分离效率。此外,
更新日期:2020-11-30
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