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Nonmonotonic crossover in electronic phase separated manganite superlattices driven by the superlattice period
Physical Review B ( IF 3.7 ) Pub Date : 2020-12-02 , DOI: 10.1103/physrevb.102.235107
Yinyan Zhu , Biying Ye , Qiang Li , Hao Liu , Tian Miao , Lijun Wu , Lei Li , Lingfang Lin , Yi Zhu , Zhe Zhang , Qian Shi , Yulong Yang , Kai Du , Yu Bai , Yang Yu , Hangwen Guo , Wenbin Wang , Xiaoshan Xu , Xiaoshan Wu , Zhicheng Zhong , Shuai Dong , Yimei Zhu , Elbio Dagotto , Lifeng Yin , Jian Shen

Studying manganite superlattices [(LCMO)2n/(PCMO)n]t made of La0.625Ca0.375MnO3 (LCMO) and Pr0.625Ca0.375MnO3 (PCMO), we found an unexpected behavior varying the period n. At small n, the ensemble is a three-dimensional ferromagnetic metal due to interfacial charge transfer. At large n, the LCMO layers dominate transport. However, rather than a smooth interpolation between these limits a sharp transport and magnetic anomaly is found at an intermediate critical PCMO thickness n*. Magnetic force microscopy reveals that the phase-separation length scale also maximizes at n* where, unexpectedly, it becomes comparable to that of the (La1yPry)0.625Ca0.375MnO3 (LPCMO) alloy. We conjecture the phenomenon originates in a disorder-related length scale: Large charge-ordered clusters as in LPCMO can only nucleate when Pr-rich regions reach a critical size related to n*.

中文翻译:

超晶格周期驱动的电子相分离锰超晶格的非单调穿越

研究锰超晶格 [劳工组织2ñ/PCMOñ]Ť 由...制成 0.6250.375Ø3 (LCMO)和 0.6250.375Ø3 (PCMO),我们发现了不同时期的意外行为 ñ。在小ñ,由于界面电荷转移,该集合是三维铁磁金属。大体上ñ,LCMO层主导着运输。但是,不是在这些限制之间进行平滑插值,而是在中间临界PCMO厚度处发现了尖锐的传输和磁异常。ñ*。磁力显微镜显示相分离长度标度在ñ* 出乎意料的是,它变得与 1个ÿÿ0.6250.375Ø3(LPCMO)合金。我们推测,这种现象起源于与疾病有关的长度尺度:LPCMO中的大型带电荷簇只能在富Pr区域达到与ñ*
更新日期:2020-12-02
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