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Auger electron wave packet interferometry on extreme timescales with coherent soft x-rays
Journal of Physics B: Atomic, Molecular and Optical Physics ( IF 1.6 ) Pub Date : 2020-11-27 , DOI: 10.1088/1361-6455/abc661
Sergey Usenko 1, 2 , David Schwickert 1 , Andreas Przystawik 1 , Karolin Baev 2 , Ivan Baev 2 , Markus Braune 1 , Lars Bocklage 1, 3 , Marie Kristin Czwalinna 1 , Sascha Deinert 1 , Stefan Dsterer 1 , Andreas Hans 4 , Gregor Hartmann 4, 5 , Christian Haunhorst 6 , Marion Kuhlmann 1 , Steffen Palutke 1 , Ralf Rhlsberger 1, 3 , Juliane Rnsch-Schulenburg 1 , Philipp Schmidt 4 , Slawomir Skruszewicz 1 , Sven Toleikis 1 , Jens Viefhaus 5 , Michael Martins 2 , Andr Knie 4 , Detlef Kip 6 , Tim Laarmann 1, 3
Affiliation  

Wave packet interferometry provides benchmark information on light-induced electronic quantum states by monitoring their relative amplitudes and phases during coherent excitation, propagation, and decay. The relative phase control of soft x-ray pulse replicas on the single-digit attosecond timescale achieved in our experiments makes this method a powerful tool to probe ultrafast quantum phenomena such as the excitation of Auger shake-up states with sub-cycle precision. In this contribution we present first results obtained for different Auger decay channels upon generating L-shell vacancies in argon atoms using Michelson-type all-reflective interferometric autocorrelation at a central free-electron laser photon energy of 274.7eV.



中文翻译:

具有相干软X射线的极端时标上的俄歇电子波包干涉测量

波包干涉测量法通过监测相干激发,传播和衰减期间的相对振幅和相位,提供有关光诱导电子量子态的基准信息。在我们的实验中,在一位数的阿秒级时间尺度上对软X射线脉冲副本的相对相位控制使该方法成为探测超快速量子现象(如具有亚循环精度的俄歇振动状态激发)的有力工具。在这项贡献中,我们介绍了在中心自由电子激光光子能量为274.7eV时,使用迈克尔逊型全反射干涉自相关技术在氩原子中产生L壳空位时在不同的俄歇衰变通道上获得的第一个结果。

更新日期:2020-11-27
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