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Controlling the Ultrafast Dynamics of HD+ by the Carrier-Envelope Phases of an Ultrashort Laser Pulse: A Quasi-Classical Dynamics Study
The Journal of Physical Chemistry A ( IF 2.9 ) Pub Date : 2020-11-16 , DOI: 10.1021/acs.jpca.0c08979
Gaurav Pandey 1 , Diptesh Dey 1 , Ashwani K. Tiwari 1
Affiliation  

A theoretical study on the coupled electron-nuclear dynamics of HD+ molecular ions under ultrashort, intense laser pulses is performed by employing a well-established quasi-classical model. The influence of the laser carrier-envelope phase on various channel (H + D+, D + H+, and H+ + D+) probabilities is investigated at different laser field intensities. The carrier-envelope phase is found to govern the dissociation (H + D+ and D + H+) and Coulomb explosion (H+ + D+) channel probabilities. The kinetic energy release distributions of the fragments are also found to be sensitive to the carrier-envelope phase of the laser pulse. Our results are in agreement with the previously reported quantum dynamics studies and experiments.

中文翻译:

通过超短激光脉冲的载波包络相位控制HD +的超快动力学:准经典动力学研究

通过建立良好的准经典模型,对超短,强激光脉冲下HD +分子离子的耦合电子核动力学进行了理论研究。研究了在不同的激光场强度下,激光载流子包络相位对各种通道(H + D +,D + H +和H + + D +)概率的影响。发现载流子-包裹体相决定了解离(H + D +和D + H +)和库仑爆炸(H + + D +)渠道概率。还发现碎片的动能释放分布对激光脉冲的载流子-包络相敏感。我们的结果与先前报道的量子动力学研究和实验一致。
更新日期:2020-11-25
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