Journal of Nuclear Materials ( IF 3.1 ) Pub Date : 2020-11-07 , DOI: 10.1016/j.jnucmat.2020.152647 Hao-Dong Liu , Hai-Shan Zhou , Li Qiao , Hong Zhang , Guang-Nan Luo
Deuterium (D) plasma-driven permeation (PDP) experiments through reduced activation ferritic/martensitic (RAFM) steel with and without tungsten (W) deposition layer have been performed. The results confirm that W deposition does not always work as D permeation barrier, but enhances D permeation flux through the structural material under certain conditions. The steady state PDP fluxes through RAFM steel with a thin (∼30 nm) W deposition layer have been found to be larger than those of bare RAFM steel, whereas the RAFM steel membrane with a thick (6.0 μm) W deposition layer exhibits lower permeation fluxes than those of bare steel sample. Tritium Migration Analysis Program (TMAP) calculation indicates that the steady state permeation flux is determined by the D concentration accumulated at the interface between W layer and RAFM steel, which is highly relevant to the W deposition thickness. Only when the W thickness is larger than ∼2 μm, the steady state permeation flux will be controlled by diffusion in W deposition layer.
中文翻译:
钨沉积厚度对RAFM钢中氢同位素渗透的影响
已通过具有和不具有钨(W)沉积层的还原活化铁素体/马氏体(RAFM)钢进行了氘(D)等离子体驱动的渗透(PDP)实验。结果证实,W沉积并不总是作为D的渗透屏障,而是在一定条件下增强了D渗透通过结构材料的通量。已经发现,穿过具有较薄(〜30 nm)W沉积层的RAFM钢的稳态PDP通量要比裸RAFM钢的稳态PDP通量大,而具有较厚(6.0μm)W沉积层的RAFM钢膜的渗透性较低。通量比裸钢样品大。Migration迁移分析程序(TMAP)的计算表明,稳态渗透通量由W层与RAFM钢之间的界面处积累的D浓度决定,这与W沉积厚度高度相关。仅当W的厚度大于〜2μm时,稳态渗透通量才由W沉积层中的扩散来控制。