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Characterization of radionuclide activity concentrations and lifetime cancer risk due to particulate matter in the Singrauli Coalfield, India
Environmental Monitoring and Assessment ( IF 3 ) Pub Date : 2020-10-06 , DOI: 10.1007/s10661-020-08619-1
Akhilesh Kumar Yadav , Philip Karl Hopke

In this study, the activities of 40K, 210Pb, 232Th, 234U, 235U, and 238U in size-segregated particulate matter (PM) were measured in the Singrauli Coalfield, India. Different isotopic compositions were found relative to natural uranium ratios. The radioactivity concentration ratios in different PM sizes [PM2.5, PM10, and suspended particulate matter (SPM)] suggested that anthropogenic sources affected the uranium isotopic compositions in the area. A different isotopic composition from the natural uranium composition was found. The correlation coefficients between the measured isotopes (40K, 210Pb, 232Th, 234U, 235U, and 238U) and meteorological factors were calculated. PM emissions were affected by the meteorological conditions, which in turn, influenced the U and Th concentrations in PM. The 232Th/238U activity ratio in particulate matter was between 0.20 and 1.54 with an average value of 0.9 ± 0.5, 0.2 to 1.1 (0.8 ± 0.7), and 0.2 to 1.2 with an average value of 0.8 ± 0.8 in PM2.5, PM10, and SPM, respectively. These range were quite different from the average crustal ratio of 3.5, indicating that the 238U concentrations were elevated in this region relative to Th. However, compared with Th, the dose contribution of U to the public was negligible. The average effective dose in public owing to inhalation of natural radioactive 40K, 210Pb, 232Th, and 234U, 235U, and 238U in the atmosphere was between 0.03 and 327 nSv year−1. These doses associated with the inhalation of particulate matter were lower than world airborne reference value as reported by UNSCEAR (2000a).



中文翻译:

印度Singrauli煤田中放射性核素活度浓度的表征和由于颗粒物引起的终生癌症风险

在这项研究中,在印度的辛格劳利煤田中测量了40 K,210 Pb,232 Th,234 U,235 U和238 U的大小分离颗粒物(PM)的活性。发现相对于天然铀比率不同的同位素组成。不同PM尺寸[PM 2.5,PM 10和悬浮颗粒物(SPM)]的放射性浓度比表明,人为源影响了该地区的铀同位素组成。发现与天然铀组成不同的同位素组成。被测同位素之间的相关系数(40 K,计算了210 Pb,232 Th,234 U,235 U和238 U)和气象因子。PM排放受气象条件的影响,而气象条件又影响PM中的U和Th浓度。在PM 2.5中,颗粒物的232 Th / 238 U活度比在0.20至1.54之间,平均值为0.9±0.5、0.2至1.1(0.8±0.7),以及0.2至1.2,平均值为0.8±0.8。PM 10和SPM分别。这些范围与3.5的平均地壳比率有很大差异,表明238相对于Th,该区域的U浓度升高。但是,与Th相比,U对公众的剂量贡献可忽略不计。在公共欠平均有效剂量天然放射性的吸入40 K,210的Pb,232 Th和234 U,235 U和238中的U气氛NSV年0.03和327之间-1。这些吸入颗粒物的剂量低于联合国航空航天研究中心(2000a)报告的世界航空参考值。

更新日期:2020-10-07
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