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Secondary electron emission by plasmon-induced symmetry breaking in highly oriented pyrolytic graphite
Physical Review Letters ( IF 8.385 ) Pub Date : 
Wolfgang S. M. Werner; Vytautas Astašauskas; Philipp Ziegler; Alessandra Bellissimo; Giovanni Stefani; Lukas Linhart; Florian Libisch

Two-particle spectroscopy with correlated electron pairs is used to establish the causal link between the secondary electron spectrum, the (π+σ)plasmon peak and the unoccupied band structure of highly oriented pyroly}tic graphite. The plasmon spectrum is resolved with respect to the involved interband transitions and clearly exhibits final state effects, in particular due to the energy gap between the interlayer resonances along the ΓA-direction. The corresponding final state effects can also be identified in the secondary electron spectrum. Interpretation of the results is performed on the basis of density functional theory and tight binding calculations. Excitation of the plasmon perturbs the symmetry of the system and leads to hybridisation of the interlayer resonances with atom-like σ* bands along the ΓA-direction. These hybrid states have a high density of states as well as sufficient mobility along the graphite c-axis leading to the sharp $$3 eV resonance in the spectrum of emitted secondary electrons reported throughout the literature. : …
更新日期:2020-09-15

 

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