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One-Dimensional Magnetic Order Stabilized in Edge-Reconstructed MoS2 Nanoribbon via Bias Voltage.
The Journal of Physical Chemistry Letters ( IF 5.7 ) Pub Date : 2020-08-19 , DOI: 10.1021/acs.jpclett.0c02302
Xiaohui Deng 1, 2 , Zhenyu Li 1 , Jinlong Yang 1
Affiliation  

Low-dimensional nanostructures are expected to play an important role in spintronics. However, in low-dimensional systems, thermal fluctuations become more significant, which makes long-range magnetic ordering thermodynamically unfavorable. For example, as predicted by the Ising model, 1D magnetic order cannot survive, even at an arbitrary low finite temperature. In this study, utilizing a nanoproximity effect, we design a MoS2 nanoribbon material to stabilize 1D magnetic order without requiring the explicit application of an external magnetic field. The designed MoS2 nanoribbon has a new edge-reconstruction pattern, which is much more stable than previously reported structures. As a novel electronic property, one edge is nonmagnetic but conductive, and the opposite edge contains a magnetic moment in the predicted reconstruction pattern. Therefore, a bias voltage can drive a current along the former edge, which then generates a magnetic field at the opposite edge to stabilize the 1D magnetic order there. This result opens a new avenue to realize the integrated electrical control of magnetism.

中文翻译:

通过偏置电压在边缘重建的MoS2纳米带中稳定的一维磁阶。

低维纳米结构有望在自旋电子学中发挥重要作用。但是,在低维系统中,热波动变得更加明显,这使长距离磁排序在热力学上不利。例如,根据伊辛(Ising)模型预测,即使在任意低的有限温度下,一维磁阶也无法幸免。在这项研究中,利用纳米邻近效应,我们设计了MoS 2纳米带材料来稳定一维磁阶,而无需明确施加外部磁场。设计的MoS 2纳米带具有新的边缘重建模式,比以前报道的结构稳定得多。作为一种新颖的电子属性,一个边缘是非磁性的,但具有导电性,而另一边缘则在预测的重构模式中包含磁矩。因此,偏置电压可以沿前一个边缘驱动电流,然后在相对的边缘上产生磁场以稳定一维磁阶。这一结果为实现磁性的集成电控制开辟了一条新途径。
更新日期:2020-09-18
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