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Investigation on sub-band gap defects aided UV to NIR broad-band low-intensity photodetection by SnO2 thin film
Sensors and Actuators A: Physical ( IF 4.6 ) Pub Date : 2020-06-16 , DOI: 10.1016/j.sna.2020.112168
Ayon Das Mahapatra , Durga Basak

We report a broad-band low-intensity photodetection enriched with a good reproducibility by SnO2 thin film grown by a facile vapour-liquid-solid technique. Unprecedentedly, simple Al/SnO2/Al photoconductive device, operated at room temperature in the wavelength range from ultraviolet (300 nm) to near infra-red (800 nm) show responsivities 2.04, 0.19, 0.25 and 0.19 mA/W respectively for 300 nm, 450 nm, 550 nm & 800 nm lights indicating broad-band photodetectivity due to its sub-band gap defects. It can also detect lights with very low-intensity of 14 μW/cm2 (300 nm), 54 μW/cm2 (450 nm), 42 μW/cm2 (550 nm) & 12 μW/cm2 (800 nm) having responsivity values of 8.00, 1.02, 1.42 and 0.70 mA/W respectively. Interestingly, the defect states within the band gap causing the photosensitivity over a wide wavelength range have been proposed uniquely by a systematic successive photocurrent transient experiment using illuminations from NIR to UV region supported by the photoluminescence results. These excellent performances unambiguously demonstrate that the simple SnO2 film is promising for utilization as efficient broad-band photodetector.



中文翻译:

SnO 2薄膜辅助UV对NIR宽带低强度光检测的亚带隙缺陷研究

我们报告了宽带低强度光电检测,通过利用便捷的液-液-固技术生长的SnO 2薄膜丰富了良好的再现性。前所未有地,简单的Al / SnO 2 / Al光电导器件在室温下从紫外(300 nm)到近红外(800 nm)的波长范围内运行,其300的响应度分别为2.04、0.19、0.25和0.19 mA / W nm,450 nm,550 nm和800 nm的光表示其子带隙缺陷,因此具有宽带光电探测性。它还可以检测强度非常低的光,分别为14μW/ cm 2(300 nm),54μW/ cm 2(450 nm),42μW/ cm 2(550 nm)和12μW/ cm 2(800 nm)的响应度分别为8.00、1.02、1.42和0.70 mA / W。有趣的是,通过系统的连续光电流瞬态实验,使用从NIR到UV区域的照明(由光致发光结果支持),独特地提出了在宽波长范围内引起光敏性的带隙内缺陷状态。这些优异的性能清楚地表明,简单的SnO 2膜有望用作有效的宽带光电探测器。

更新日期:2020-06-16
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