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g‐C3N4/TiO2 Composite Film in the Fabrication of a Photocatalytic Air‐Purifying Pavements
Solar RRL ( IF 7.9 ) Pub Date : 2020-05-27 , DOI: 10.1002/solr.202000170
Yu Huang 1, 2, 3 , Jing Zhang 1 , Zhenyu Wang 1 , Yan Liu 1 , Pengge Wang 1 , Jun-ji Cao 1, 2, 3 , Wingkei Ho 4
Affiliation  

The fabrication of a photocatalytic air‐purifying pavement with a facile loading route, long depolluting period, and excellent deNOx activity under weak solar irradiation is essential for ambient air purification. Herein, a promising methodology is developed relying on the exploitation of a graphitic carbon nitride/TiO2 (g‐C3N4/TiO2) composite hydrosol at room temperature. The TiO2 hydrosol can act as a source of photocatalyst and dispersant for g‐C3N4 during loading. The photoinduced hydrophilicity, adhesive force, and regeneration tests in the laboratory show the long‐term deNOx application potential of g‐C3N4/TiO2 coatings. Field studies indicate that the NO removal rate is 70.7% of g‐C3N4/TiO2‐coated pavement in the morning (07:00–10:00) and afternoon (17:00–19:00), at which times solar radiation is weakest. The deNOx efficiency is influenced by solar irradiation and traffic volume. The latter exerts a more significant influence on deNOx efficiency than the former. A desirable route in fabricating a photocatalytic air‐purifying pavement is provided and offers a promising photocatalyst suitable for outdoor environmental remediation.

中文翻译:

g-C3N4 / TiO2复合膜在光催化空气净化路面的制备中

用容易装载路线,长周期消除污染,以及优异的DENO光催化剂的空气净化路面的制造X活动弱太阳能照射下为环境空气净化必要的。在此,依靠在室温下开发石墨氮化碳/ TiO 2(g-C 3 N 4 / TiO 2)复合水溶胶,开发了一种有前途的方法。TiO 2溶胶可以在装载过程中充当g‐C 3 N 4的光催化剂和分散剂。光致亲水性,附着力,并在实验室再生试验表明长期DENO Xg‐C 3 N 4 / TiO 2涂层的应用潜力。现场研究表明,在早上(07:00-10:00)和下午(17:00-19:00),g-C 3 N 4 / TiO 2涂层路面的NO去除率为70.7%。太阳辐射最弱。所述DENO X效率是由太阳能电池照射和交通量的影响。后者发挥上DENO更显著影响X效率高于前者。提供了制造光催化空气净化路面的理想途径,并提供了一种有前途的光催化剂,适用于室外环境修复。
更新日期:2020-05-27
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