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Spatially separating redox centers on 2D carbon nitride with cobalt single atom for photocatalytic H2O2 production [Engineering]
Proceedings of the National Academy of Sciences of the United States of America ( IF 9.580 ) Pub Date : 2020-03-24
Chiheng Chu, Qianhong Zhu, Zhenhua Pan, Srishti Gupta, Dahong Huang, Yonghua Du, Seunghyun Weon, Yueshen Wu, Christopher Muhich, Eli Stavitski, Kazunari Domen, Jae-Hong Kim

Redox cocatalysts play crucial roles in photosynthetic reactions, yet simultaneous loading of oxidative and reductive cocatalysts often leads to enhanced charge recombination that is detrimental to photosynthesis. This study introduces an approach to simultaneously load two redox cocatalysts, atomically dispersed cobalt for improving oxidation activity and anthraquinone for improving reduction...
更新日期:2020-03-26

 

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