Abstract

The review presents an overview of studies in the surface science of oxide and related surfaces with an emphasis of the studies performed in the authors’ group. Novel instruments and technique developments, as well as their applications are reported, in an attempt to cover studies on model systems of increasing complexity, including some of the key ingredients of an industrially applied heterogeneous catalyst and its fabrication. The review is intended to demonstrate the power of model studies in understanding heterogeneous catalysis at the atomic level. The studies include those on supported nano-particles, both, prepared in vacuum and from solution, interaction of surfaces and the underlying bulk with molecules from the gas phase, strong metal support interaction, as well as the first attempt to include studies on reactions in confined spaces.

中文翻译：

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在原子级的非均相催化中的章节模型系统：个人观点

摘要

这篇综述概述了氧化物和相关表面的表面科学研究，并着重于作者小组中进行的研究。为了涵盖对日益复杂的模型系统的研究，包括工业应用的非均相催化剂及其制造的一些关键成分，试图报道新颖的仪器和技术发展及其应用。该综述旨在证明模型研究在理解原子级非均相催化方面的作用。这些研究包括在真空中和从溶液中制备的负载型纳米颗粒的研究，表面和下面的主体与气相分子的相互作用，强金属载体的相互作用，以及首次尝试包括密闭空间。