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Proton Insertion Chemistry of a Zinc-Organic Battery.
Angewandte Chemie International Edition ( IF 12.959 ) Pub Date : 2020-01-14 , DOI: 10.1002/anie.201916529
Zhiwei Tie,Luojia Liu,Shenzhen Deng,Dongbing Zhao,Zhiqiang Niu

Proton storage in rechargeable aqueous zinc-ion batteries (ZIBs) is attracting extensive attention owing to the fast kinetics of H+ insertion/extraction. However, it has not been achieved in organic materials-based ZIBs with a mild electrolyte. Now, aqueous ZIBs based on diquinoxalino [2,3-a:2',3'-c] phenazine (HATN) in a mild electrolyte are developed. Electrochemical and structural analysis confirm for the first time that such Zn-HATN batteries experience a H+ uptake/removal behavior with highly reversible structural evolution of HATN. The H+ uptake/removal endows the Zn-HATN batteries with enhanced electrochemical performance. Proton insertion chemistry will broaden the horizons of aqueous Zn-organic batteries and open up new opportunities to construct high-performance ZIBs.
更新日期:2020-02-14

 

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