李正全,男,1979年3月生,浙江师范大学“双龙学者”特聘教授、博士生导师、硕士生导师。现任浙江师范大学化学与材料科学学院院长,光电子研究院副院长。2000年毕业于安徽大学化学化工学院,获工学学士学位。2005年毕业于中国科学技术大学化学系,获理学博士学位。随后,分别在新加坡国立大学和美国华盛顿大学从事博士后研究。2009年在浙江师范大学开始教学与科研工作。长期从事无机纳米材料的合成、改性及应用领域的研究工作,已在国际期刊《Angew. Chem. Int. Ed.》、《Adv. Mater.》、《Nano Lett.》、《ACS Nano》、《ACS Energy Lett.》等上以第一作者或通讯作者发表论文140余篇,论文引用次数累计超过10000余次,单篇最高引用870次,先后有18篇论文入选高被引论文,部分研究成果曾被其他国际刊物或网站评为研究亮点。入选全球前10万名学者名单和全球前2%顶尖科学家榜单,获得多项国家自然科学基金项目和浙江省杰青项目等资助
主要科研项目:
1. 国家自然科学基金(面上项目):上转换/MOF复合纳米材料的可控合成与衍生、表面物种调控及其NIR光氧化性能研究,在研;
2. 国家自然科学基金(面上项目):上转换纳米光触媒及纳米药物的设计、合成与性能研究,已结题;
3. 国家自然科学基金(青年基金):用于光动力治疗和智能药物输运的纳米上转换荧光材料的构建和性能研究,已结题;
4. 国家重点研发计划重点专项子课题:微纳电子制造用超高纯电子气体:ppb级气体杂质和金属离子检测技术研究,已结题;
5. 浙江省自然科学基金(重点项目):近红外光响应的钙钛矿量子点/WOx复合材料的合成及其光催化CO2还原性能研究,在研;
6. 浙江省钱江人才计划项目:上转换纳米荧光材料的友好合成、表面改性及生物医学应用研究,已结题;
7. 浙江省自然科学基金(杰青项目):红外响应的上转换/半导体复合纳米材料的设计、合成及催化性能研究,已结题;
8. 浙江省自然科学基金(面上项目):NaYF4/TiO2复合纳米材料的组装和性能研究,已结题。
部分代表性论文(2009年至今):
52. Y. Wang, J. Wang*, M. Zhang, S. Zheng, J. Wu, T. Zheng, G. Jiang, and Z. Q. Li* In Situ Constructed Perovskite–Chalcogenide Heterojunction for Photocatalytic CO2 Reduction Small, 2023, 2300841.
51. S. M. Li, J. Y. Wang, X. Y. Lv, S. Zheng, J. Wang, Z. Q. Li,* Controllable synthesis of MOFs-derived porous and tubular bimetallic Fe-Ni phosphides for efficient electrocatalytic water splitting. Catal. Sci. Technol. 2023, 13, 1512.
50. X. Zhong, X. Liang, X. Lin, J. Wang*, M. Z. Shahid*, and Z. Q. Li* A New 0D-2D CsPbBr3-Co3O4 Heterostructure Photocatalyst with Efficient Charge Separation for Photocatalytic CO2 Reduction. Inorg. Chem. Front., 2023, 10.1039/D3QI00527E.
49. J. Wang,* Y. Y. Shi, Y. H. Wang, Z. Q. Li,* Rational design of metal halide perovskite nanocrystals for photocatalytic CO2 reduction: recent advances, challenges, and prospects. ACS Energy Lett. 2022, 7, 2043. (高被引论文)
48. N. Y. Li, X. J. Chen, J. Wang,* X. M. Liang, L. T. Ma, X. L. Jing, D. L. Chen,* Z. Q. Li,* ZnSe nanorods-CsSnCl3 perovskite heterojunction composite for photocatalytic CO2 reduction. ACS Nano. 2022, 16, 3332. (高被引论文)
47. S. M. Li, F. Wu, R. B. Lin, J. Wang, C. X. Li, Z. Q. Li,* J. Jiang,* Y. J. Xiong,* Enabling photocatalytic hydrogen production over Fe-based MOFs by refining band structure with dye sensitization. Chem. Eng. J. 2022, 429, 132217.
46. A. M. Idris, S. Zheng, L. J. Wu, S. Zhou, H. Lin, Z. H. Chen, L. Y. Xu, J. Wang, Z. Q. Li,* A heterostructure of halide and oxide double perovskites Cs2AgBiBr6/Sr2FeNbO6 for boosting the charge separation toward high efficient photocatalytic CO2 reduction under visible-light irradiation. Chem. Eng. J. 2022, 446, 137139
45. Q. Zheng, J. Wang,* X. Li, Y. Bai, Y. P. Li, J. C. Wang, Y. Y. Shi, X. Y. Jiang, Z. Q. Li,* Surface halogen compensation on CsPbBr3 nanocrystals with SOBr2 for photocatalytic CO2 reduction. ACS Mater. Lett. 2022, 4, 1638.
44. X. Y. Jiang, Y. X. Ding, S. Zheng, Y. L. Ye, Z. Q. Li,* L. Y. Xu, J. Wang, Z. B. Li, X. J. Loh, Y. E. Ye,* L. C. Sun,* In-situ generated CsPbBr3 nanocrystals on O-defective WO3 for photocatalytic CO2 reduction. ChemSusChem 2022, 15, e202102295 (高被引论文)
43. J. Wang,* L. Xiong, Y. Bai, Z. J. Chen, Q. Zheng, Y. Y. Shi, C. Zhang, G. C. Jiang, Z. Q. Li,* Mn-doped perovskite nanocrystals for photocatalytic CO2 reduction: Insight into the role of the charge carriers with prolonged lifetime. Sol. RRL 2022, 6, 2200294.
42. C. Zhang, W. Zhang, F. Karadas, J. X. Low, R. Long, C. H. Liang,* J. Wang, Z. Q. Li,* Y. J. Xiong,* Laser-ablation assisted strain engineering of gold nanoparticles for selective electrochemical CO2 reduction. Nanoscale. 2022, 14, 7702.
41. J. Wang,* J. L. Liu, Z. L. Du,* Z. Q. Li,* Recent advances in metal halide perovskite photocatalysts: properties, synthesis and applications. J. Energy Chem. 2021, 54, 770.
40. Q. Wang, J. W,* J. C. Wang, X. Hu, Y. Bai, X. H. Zhong, Z. Q. Li,* Coupling CsPbBr3 quantum dots with covalent triazine frameworks for visible-light-driven CO2 reduction. ChemSusChem. 2021, 14, 1131.
39. J. C. Wang, N. Y. Li, A. M. Idris, J. Wang,* X. Y. Du, Z. X. Pan, Z. Q. Li,* Surface defect engineering of CsPbBr3 nanocrystals for high efficient photocatalytic CO2 reduction. Sol. RRL 2021, 5, 2100154
38. M. Zhang, X. J. Chen, X. Y. Jiang, J. Wang,* L. Y. Xu, J. H. Qiu, W. R. Lu, D. L. Chen,* Z. Q. Li,* Activate Fe3S4 nanorods by Ni doping for efficient dye-sensitized photocatalytic hydrogen production. ACS Appl. Mater. Interfaces 2021, 13, 14198.
37. S. M. Li, J. Tan, Z. J. Jiang, J. Wang, Z. Q. Li,* MOF-derived bimetallic Fe-Ni-P nanotubes with tunable compositions for dye-sensitized photocatalytic H2 and O2 production. Chem. Eng. J 2020, 384, 123354.
36. J. C. Wang, J. Wang,* N. Y. Li, X. Y. Du, J. Ma, C. H. He, Z. Q. Li,* Direct z-scheme 0D/2D heterojunction of CsPbBr3 quantum dots/Bi2WO6 nanosheets for efficient photocatalytic CO2 reduction. ACS Appl. Mater. Interfaces 2020, 12, 31477. (高被引论文)
35. S. M. Li, K. Ji, M. Zhang, C. S. He, J. Wang, Z. Q. Li,* Boosting the photocatalytic CO2 reduction of metal-organic frameworks by encapsulating carbon dots. Nanoscale. 2020, 12, 9533.
34. Z. J. Chen, Y. G. Hu, J. Wang,* Q. Shen, Y. H. Zhang, C. Ding, Y. Bai, G. C. Jiang, N. Gaponik, Z. Q. Li,* Boosting photocatalytic CO2 reduction on CsPbBr3 perovskite nanocrystals by immobilizing metal complexes. Chem. Mater. 2020, 32, 1517. (高被引论文)
33. M. Wang, D. M. Wang, Q. Chen, C. X. Li,* Z. Q. Li,* J. Lin,* Recent advances in glucose-oxidase-based nanocomposites for tumor therapy. Small 2019, 15, 1903895.
32. J. Y. Wang, S. M. Li, R. B. Lin, G. M. Tu, J. Wang, Z. Q. Li,* MOF-derived hollow β-FeOOH polyhedra anchored with α-Ni(OH)2 nanosheets as efficient electrocatalysts for oxygen evolution. Electrochim. Acta 2019, 301, 258.
31. R. B. Lin, S. M. Li, J. Y. Wang, J. P. Xu, C. H. Xu, J. Wang, C. X. Li, Z. Q. Li,* Facile generation of carbon quantum dots in MIL-53(Fe) particles as localized electron acceptors for enhancing their photocatalytic Cr(VI) reduction. Inorg. Chem. Front. 2018, 5, 3170.
30. C. X. Li, L. L. Xu, Z. H. Liu, Z. Q. Li,* Z. W. Quan, A. A. Al Kheraif, J. Lin,* Current progress in the controlled synthesis and biomedical applications of ultrasmall (<10 nm) NaREF4 nanoparticles. Dalton Trans. 2018, 47, 8538.
29. B. X. Li,* L. Z. Shao, R. S. Wang, X. P. Dong,* F. G. Zhao,* P. Gao, Z. Q. Li,* Interfacial synergism of Pd-decorated BiOCl ultrathin nanosheets for the selective oxidation of aromatic alcohols. J. Mater. Chem. A 2018, 6, 6344.
28. J. Y. Wang, C. Cui, R. B. Lin, C. H. Xu, J. Wang, Z. Q. Li,* Hybrid cobalt-based electrocatalysts with adjustable compositions for electrochemical water splitting derived from Co2+-Loaded MIL-53(Fe) particles. Electrochim. Acta 2018, 286, 397.
27. C. Cui, J. Y. Wang, Z. G. Lou, J. Wang, C. X. Li, Z. Q. Li,* MOF-mediated synthesis of monodisperse Co(OH)2 flower-like nanosheets for enhanced oxygen evolution reaction. Electrochim. Acta 2018, 273, 327.
26. M. H. Li, Z. J. Zheng, Y. Q. Zheng, C. Cui, C. X. Li,* Z. Q. Li,* Controlled growth of metal–organic framework on upconversion nanocrystals for NIR-enhanced photocatalysis. ACS Appl. Mater. Interfaces 2017, 9, 2899.
25. C. Cui, M. J. Tou, M. H. Li, Z. G. Lou, L. B. Xiao, S. Bai, Z. Q. Li,* Heterogeneous semiconductor shells sequentially coated on upconversion nanoplates for NIR-light enhanced photocatalysis. Inorg. Chem. 2017, 56, 2328.
24. Y. Z. Zhu, C. Gao. S. Bai, S. M. Chen, R. Long, L. Song, Z. Q. Li,* Y. J. Xiong,* Hydriding Pd cocatalysts: an approach to giant enhancement on photocatalytic CO2 reduction into CH4. Nano Res. 2017, 10, 3396.
23. M. H. Li, J. Wang, Y. Q. Zheng, Z. J. Zheng, C. X. Li, Z. Q. Li,* Anchoring NaYF4:Yb,Tm upconversion nanocrystals on concave MIL-53(Fe) octahedra for NIR-light enhanced photocatalysis. Inorg. Chem. Front. 2017, 4, 1757.
22. K. Wang, W. L. Qincheng, F. Y. Wang, S. Bai, S. Li, Z. Q. Li,* Coating a N-doped TiO2 shell on dually sensitized upconversion nanocrystals to provide NIR-enhanced photocatalysts for efficient utilization of upconverted emissions. Inorg. Chem. Front. 2016, 3, 1190.
21. M. J. Tou, Y. Y. Mei, S. Bai,* Z. G. Luo, Y. Zhang, Z. Q. Li,* Depositing CdS nanoclusters on carbon-modified NaYF4:Yb,Tm upconversion nanocrystals for NIR-light enhanced photocatalysis. Nanoscale 2016, 8, 553.
20. L. J. Bai, W. Y Jiang, C. X. Gao, S. X. Zhong, L. H. Zhao, S. Bai,* Z. Q. Li,* Facet engineered interface design of NaYF4:Yb, Tm upconversion nanocrystals on BiOCl nanoplates for enhanced near-infrared photocatalysis. Nanoscale 2016, 8, 19014.
19. W. J. Yin, S. Bai, Y. J. Zhong, Z. Q. Li,* Y. Xie, Direct generation of fine Bi2WO6 nanocrystals on g-C3N4 nanosheets for enhanced photocatalytic activity. ChemNanoMat 2016, 2, 732.
18. W. J. Yin, L. J. Bai, Y. Z. Zhu, S. X. Zhong, L. H. Zhao, Z. Q. Li,* S. Bai,* Embedding metal in the interface of a p-n heterojunction with a stack design for superior z-scheme photocatalytic hydrogen evolution. ACS Appl. Mater. Interfaces. 2016, 8, 23133.
17. S. Q. Zhou, S. Bai,* E. J. Cheng, R. Qiao, Y. Xie, Z. Q. Li,* Facile 'embedding' of Au nanocrystals into silica spheres with controllable quantity for improved catalytic reduction of p-nitrophenol. Inorg. Chem. Front. 2015, 2, 938.
16. L. Li, S. Q. Zhou, E. J. Chen, R. Qiao, Y. J. Zhong, Y. Zhang, Z. Q. Li,* Simultaneous formation of silica-protected and N-doped TiO2 hollow spheres using organic-inorganic silica as self-removed templates. J. Mater. Chem. A. 2015, 3, 2234.
15. W. K. Su, M. M. Zheng, L. Li, K. Wang, R. Qiao,* Y. J. Zhong, Y. Hu, Z. Q. Li,* Directly coat TiO2 on hydrophobic NaYF4:Yb,Tm nanoplates and regulate their photocatalytic activities with the core size. J. Mater. Chem. A. 2014, 2, 13486.
14. L. Y. Bao, H. L. You, L. M. Wang, L. Li, R. Qiao, Y. Zhang, Y. J. Zhong, Y. J. Xiong, Z. Q. Li,* Self-assembly of LaF3:Yb,Er/Tm nanoplates into colloidal spheres and tailoring their upconversion emissions with fluorescent dyes. J. Mater. Chem. C. 2014, 2, 8949.
13. Z. Q. Li,* C. L. Li, Y. Y. Mei, L. M. Wang, G. H. Du, Y. J. Xiong, Synthesis of rhombic hierarchical YF3 nanocrystals and their use as upconversion photocatalysts after TiO2 coating. Nanoscale 2013, 5, 3030.
12. Y. B. Zeng, Z. Q. Li,* Y. F. Liang, X. Q. Gan, M. M. Zheng, A general approach to spindle-assembled lanthanide borate nanocrystals and their photoluminescence upon Eu3+/Tb3+ doping. Inorg. Chem. 2013, 52, 9590.
11. Y. J. Zhang, F. Zheng, T. L. Yang, W. Zhou, Y. Liu, N. Man, L. Zhang, N. Jin, Q. Q. Dou, Y. Zhang, Z. Q. Li, L. P. Wen,* Tuning the autophagy-inducing activity of lanthanide-based nanocrystals through specific surface-coating peptides. Nat. Mater. 2012, 11, 817.
10. Z. Q. Li,* L. Wang, Z. Wang, X. Liu, Y. Xiong,* Modification of NaYF4:Yb,Er@SiO2 Nanoparticles with Gold Nanocrystals for Tunable Green-to-Red Upconversion Emissions. J. Phys. Chem. C 2011, 115, 3291.
9. Z. Q. Li, Y. Zhang,* Facile synthesis of lanthanide nanoparticles with paramagnetic, down- and up-conversion properties. Nanoscale, 2010, 2 1240.
2009年之前:
8. Z. Q. Li, W. Y. Li, P. H. C. Camargo, Y. N. Xia,* Facile Synthesis of Branched An Nanostructures by Templating Against a Self-destructive Lattice of Magnetic Fe Nanoparticles. Angew. Chem. Int. Ed. 2008, 47, 9653.
7.Z. Q. Li, J. Tao, X. M. Lu, W. Y. Li, X. F. Lu, Y. M. Zhu, Y. N. Xia,* Facile Synthesis of Ultrathin Gold Nanorods by Aging Iron Nanoparticles with AuCl(oleylamine) Complex in Chloroform. Nano Lett. 2008, 8, 3052.
6. Z. Q. Li, S. Jiang, Y. Zhang,* Multi-color Core-shell Structured Upconversion Fluorescent Nanoparticles. Adv. Mater. 2008, 20, 4765. (Most cited paper, citations 801)
5. Z. Q. Li, Y. Zhang,* Monodisperse Silica Coated PVP/NaYF4 Nanocrystals with Multicolor Upconversion Fluorescence Emission Angew. Chem. Int. Ed. 2006, 45, 7732. (Most cited paper)
4. Z. Q. Li, Y. Ding, Y. J. Xiong, Q. Yang, Y. Xie,* One-step Solution-based Catalytic Route to Fabricate Novel a-MnO2 Hierarchical Structures in Large-scale. Chem. Commun. 2005, 918. (Most cited paper)
3. Z. Q. Li, Y. Ding, Y. Xiong, Y. Xie, Rational Growth of Various α-MnO2 Hierarchical Structures and β-MnO2 Nanorods via a Homogeneous Catalytic Route. Cryst. Growth Des. 2005, 5, 1953–1958.
2. Z. Q. Li, Y. Ding, Y. Xiong, Q. Yang, Y. Xie, Room-temperature surface-erosion route to ZnO nanorod arrays and urchin-like assemblies. Chem. Eur. J. 2004, 10, 5823
1. Z. Q. Li, Y. J. Xiong, Y. Xie,* Selected-control Synthesis of ZnO Nanowires and Nanorods via a PEG-assisted Route. Inorg. Chem. 2003, 42, 8105. (Most cited paper)