Longitudinal and transverse mobilities of n-type monolayer transition metal dichalcogenides in the presence of proximity-induced interactions at low temperature

J. Liu, W. Xu, Y. M. Xiao, L. Ding, H. W. Li, B. Van Duppen, M. V. Milošević, and F. M. Peeters
Phys. Rev. B 109, 195418 – Published 8 May 2024

Abstract

We present a detailed theoretical investigation on the electronic transport properties of n-type monolayer (ML) transition metal dichalcogenides (TMDs) at low temperature in the presence of proximity-induced interactions such as Rashba spin-orbit coupling (RSOC) and the exchange interaction. The electronic band structure is calculated by solving the Schrödinger equation with a k·p Hamiltonian, and the electric screening induced by electron-electron interaction is evaluated under a standard random phase approximation approach. In particular, the longitudinal and transverse or Hall mobilities are calculated by using a momentum-balance equation derived from a semiclassical Boltzmann equation, where the electron-impurity interaction is considered as the principal scattering center at low temperature. The obtained results show that the RSOC can induce the in-plane spin components for spin-split subbands in different valleys, while the exchange interaction can lift the energy degeneracy for electrons in different valleys. The opposite signs of Berry curvatures in the two valleys would introduce opposite directions of Lorentz force on valley electrons. As a result, the transverse currents from nondegenerate valleys can no longer be canceled out so that the transverse current or Hall mobility can be observed. Interestingly, we find that at a fixed effective Zeeman field, the lowest spin-split conduction subband in ML-TMDs can be tuned from one in the K-valley to one in the K-valley by varying the Rashba parameter. The occupation of electrons in different valleys also varies with changing carrier density. Therefore, we can change the magnitude and direction of the Hall current by varying the Rashba parameter, effective Zeeman field, and carrier density by, e.g., the presence of a ferromagnetic substrate and/or applying a gate voltage. By taking the ML-MoS2 as an example, these effects are demonstrated and examined. The important and interesting theoretical findings can be beneficial to experimental observation of the valleytronic effect and to gaining an in-depth understanding of the ML-TMD systems in the presence of proximity-induced interactions.

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  • Received 30 October 2023
  • Revised 11 March 2024
  • Accepted 29 April 2024

DOI:https://doi.org/10.1103/PhysRevB.109.195418

©2024 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

J. Liu1, W. Xu1,2,3,*, Y. M. Xiao1,†, L. Ding1, H. W. Li2, B. Van Duppen4, M. V. Milošević4, and F. M. Peeters2,4

  • 1School of Physics and Astronomy and Yunnan Key Laboratory of Quantum Information, Yunnan University, Kunming 650091, China
  • 2Micro Optical Instruments Inc., Shenzhen 518118, China
  • 3Key Laboratory of Materials Physics, Institute of Solid State Physics, HFIPS, Chinese Academy of Sciences, HFIPS, Hefei 230031, China
  • 4Department of Physics, University of Antwerp, Groenenborgerlaan 171, B-2020 Antwerpen, Belgium

  • *wenxu_issp@aliyun.com
  • yiming.xiao@ynu.edu.cn

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Vol. 109, Iss. 19 — 15 May 2024

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