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Catalyst: Curtailing the scalable supply of fentanyl by using chemical AI Chem (IF 23.5) Pub Date : 2024-04-23 Barbara Mikulak-Klucznik, Tomasz Klucznik, Wiktor Beker, Martyna Moskal, Bartosz A. Grzybowski
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Conjugated ladder polymers: Advances from syntheses to applications Chem (IF 23.5) Pub Date : 2024-04-23 James Shao-Jiun Yang, Lei Fang
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Reaction: Don’t hate the player in chemical AI; hate the game Chem (IF 23.5) Pub Date : 2024-04-23 Gordon Broderick
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Reaction: Navigating the promises and perils of AI-powered drug synthesis Chem (IF 23.5) Pub Date : 2024-04-23 Rick A. Bright
Rick Bright is the chief executive of Bright Global Health and former deputy assistant secretary for preparedness and response and director of BARDA at the US Department of Health and Human Services. An international expert in biodefense, emergency preparedness, pharmaceutical innovation, and public health, Dr. Bright is a member of the Council on Foreign Relations, senior fellow of the Foreign Policy
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Coral -Inspired Terahertz–Infrared Bi-Stealth Electronic Skin Angew. Chem. Int. Ed. (IF 16.6) Pub Date : 2024-04-23 Shangjing Li, Kaichao Pan, Jiang Du, Zunfeng Liu, Jun Qiu
The development of electronic skin with dual stealth functionality is crucial for enabling devices to operate effectively in dynamic electromagnetic environments, thereby facilitating intelligent electromagnetic protection for autonomous perception. However, achieving compatibility between terahertz (THz) and infrared (IR) stealth technologies remains largely unexplored due to their inherent contradictions
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Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling Angew. Chem. Int. Ed. (IF 16.6) Pub Date : 2024-04-21 Jiayou Feng, Jindi Duan, Chin-Te Hung, Zhenghao Zhang, Kailin Li, Yan Ai, Chaochao Yang, Yiyue Zhao, Zhengmin Yu, Yahong Zhang, Liang Wang, Dongyuan Zhao, Wei Li
Catalytic upcycling of polyolefins into high-value chemicals represents the direction in end-of-life plastics valorization, but poses great challenges. Here, we report the synthesis of a tandem porous catalyst via a micelle cascade assembly strategy for selectively catalytic cracking of polyethylene into olefins at a low temperature. A hierarchically porous silica layer from mesopore to macropore is
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Cyclodextrin ‘Chaperones’ Enable Quasi-Ideal Supramolecular Network Formation and Enhanced Photodimerization of Hydrophobic, Red-shifted Photoswitches in Water Angew. Chem. Int. Ed. (IF 16.6) Pub Date : 2024-04-19 Daniel Hoenders, Simon Ludwanowski, Christopher Barner-Kowollik, Andreas Walther
Precision-engineered light-triggered hydrogels are important for a diversity of applications. However, fields such as biomaterials require wavelength outside the harsh UV regime to prevent photodamage, typically requiring chromophores with extended p-conjugation that suffer from poor water solubility. Herein, we demonstrate how cyclodextrins can be used as auxiliary agents to not only solubilize such
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Discovery of (±)-Penindolenes Reveals an Unusual Indole Ring Cleavage Pathway Catalyzed by P450 Monooxygenase Angew. Chem. Int. Ed. (IF 16.6) Pub Date : 2024-04-18 Ling-Hong Meng, Takayoshi Awakawa, Xiao-Ming Li, Zhiyang Quan, Sui-Qun Yang, Bin-Gui Wang, Ikuro Abe
(±)-Penindolenes A–D (1–4), the first representatives of indole terpenoids featuring a γ-lactam skeleton, were isolated from the mangrove-derived endophytic fungus Penicillium brocae MA-231. Our bioactivity tests revealed their potent antimicrobial and acetylcholinesterase inhibitory activities. The biosynthetic reactions by the five enzymes PbaABCDE leading to γ-lactam ring formation were identified
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Dynamic acoustic optimization of pulse tube refrigerators for rapid cooldown Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Ryan Snodgrass, Vincent Kotsubo, Scott Backhaus, Joel Ullom
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Measuring statistics-induced entanglement entropy with a Hong–Ou–Mandel interferometer Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Gu Zhang, Changki Hong, Tomer Alkalay, Vladimir Umansky, Moty Heiblum, Igor Gornyi, Yuval Gefen
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Targeting NRAS via miR-1304-5p or farnesyltransferase inhibition confers sensitivity to ALK inhibitors in ALK-mutant neuroblastoma Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Perla Pucci, Liam C. Lee, Miaojun Han, Jamie D. Matthews, Leila Jahangiri, Michaela Schlederer, Eleanor Manners, Annabel Sorby-Adams, Joshua Kaggie, Ricky M. Trigg, Christopher Steel, Lucy Hare, Emily R. James, Nina Prokoph, Stephen P. Ducray, Olaf Merkel, Firkret Rifatbegovic, Ji Luo, Sabine Taschner-Mandl, Lukas Kenner, G. A. Amos Burke, Suzanne D. Turner
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An isolable, chelating bis[cyclic (alkyl)(amino)carbene] stabilizes a strongly bent, dicoordinate Ni(0) complex Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Braulio M. Puerta Lombardi, Morgan R. Faas, Daniel West, Roope A. Suvinen, Heikki M. Tuononen, Roland Roesler
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In situ captured antibacterial action of membrane-incising peptide lamellae Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Kamal el Battioui, Sohini Chakraborty, András Wacha, Dániel Molnár, Mayra Quemé-Peña, Imola Cs. Szigyártó, Csenge Lilla Szabó, Andrea Bodor, Kata Horváti, Gergő Gyulai, Szilvia Bősze, Judith Mihály, Bálint Jezsó, Loránd Románszki, Judit Tóth, Zoltán Varga, István Mándity, Tünde Juhász, Tamás Beke-Somfai
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Ocean cavity regime shift reversed West Antarctic grounding line retreat in the late Holocene Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Daniel P. Lowry, Holly K. Han, Nicholas R. Golledge, Natalya Gomez, Katelyn M. Johnson, Robert M. McKay
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Brightness illusions drive a neuronal response in the primary visual cortex under top-down modulation Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Alireza Saeedi, Kun Wang, Ghazaleh Nikpourian, Andreas Bartels, Nikos K. Logothetis, Nelson K. Totah, Masataka Watanabe
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A genomic basis of vocal rhythm in birds Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Matteo Sebastianelli, Sifiso M. Lukhele, Simona Secomandi, Stacey G. de Souza, Bettina Haase, Michaella Moysi, Christos Nikiforou, Alexander Hutfluss, Jacquelyn Mountcastle, Jennifer Balacco, Sarah Pelan, William Chow, Olivier Fedrigo, Colleen T. Downs, Ara Monadjem, Niels J. Dingemanse, Erich D. Jarvis, Alan Brelsford, Bridgett M. vonHoldt, Alexander N. G. Kirschel
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Freshwater genome-reduced bacteria exhibit pervasive episodes of adaptive stasis Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Lucas Serra Moncadas, Cyrill Hofer, Paul-Adrian Bulzu, Jakob Pernthaler, Adrian-Stefan Andrei
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Dualistic insulator states in 1T-TaS2 crystals Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Yihao Wang, Zhihao Li, Xuan Luo, Jingjing Gao, Yuyan Han, Jialiang Jiang, Jin Tang, Huanxin Ju, Tongrui Li, Run Lv, Shengtao Cui, Yingguo Yang, Yuping Sun, Junfa Zhu, Xingyu Gao, Wenjian Lu, Zhe Sun, Hai Xu, Yimin Xiong, Liang Cao
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Atomic-scale observation of localized phonons at FeSe/SrTiO3 interface Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Ruochen Shi, Qize Li, Xiaofeng Xu, Bo Han, Ruixue Zhu, Fachen Liu, Ruishi Qi, Xiaowen Zhang, Jinlong Du, Ji Chen, Dapeng Yu, Xuetao Zhu, Jiandong Guo, Peng Gao
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Boosting thermoelectric performance of single-walled carbon nanotubes-based films through rational triple treatments Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Yuan-Meng Liu, Xiao-Lei Shi, Ting Wu, Hao Wu, Yuanqing Mao, Tianyi Cao, De-Zhuang Wang, Wei-Di Liu, Meng Li, Qingfeng Liu, Zhi-Gang Chen
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Pathway-divergent coupling of 1,3-enynes with acrylates through cascade cobalt catalysis Nat. Commun. (IF 16.6) Pub Date : 2024-04-23 Heng Wang, Xiaofeng Jie, Qinglei Chong, Fanke Meng
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Prospective de novo drug design with deep interactome learning Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Kenneth Atz, Leandro Cotos, Clemens Isert, Maria Håkansson, Dorota Focht, Mattis Hilleke, David F. Nippa, Michael Iff, Jann Ledergerber, Carl C. G. Schiebroek, Valentina Romeo, Jan A. Hiss, Daniel Merk, Petra Schneider, Bernd Kuhn, Uwe Grether, Gisbert Schneider
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Highly efficient anion exchange membrane water electrolyzers via chromium-doped amorphous electrocatalysts Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Sicheng Li, Tong Liu, Wei Zhang, Mingzhen Wang, Huijuan Zhang, Chunlan Qin, Lingling Zhang, Yudan Chen, Shuaiwei Jiang, Dong Liu, Xiaokang Liu, Huijuan Wang, Qiquan Luo, Tao Ding, Tao Yao
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Tyrosine phosphorylation of CARM1 promotes its enzymatic activity and alters its target specificity Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Hidehiro Itonaga, Adnan K. Mookhtiar, Sarah M. Greenblatt, Fan Liu, Concepcion Martinez, Daniel Bilbao, Masai Rains, Pierre-Jacques Hamard, Jun Sun, Afoma C. Umeano, Stephanie Duffort, Chuan Chen, Na Man, Gloria Mas, Luca Tottone, Tulasigeri Totiger, Terrence Bradley, Justin Taylor, Stephan Schürer, Stephen D. Nimer
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Intracellular magnesium optimizes transmission efficiency and plasticity of hippocampal synapses by reconfiguring their connectivity Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Hang Zhou, Guo-Qiang Bi, Guosong Liu
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An estrogen receptor α-derived peptide improves glucose homeostasis during obesity Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Wanbao Yang, Wen Jiang, Wang Liao, Hui Yan, Weiqi Ai, Quan Pan, Wesley A. Brashear, Yong Xu, Ling He, Shaodong Guo
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Biomolecular condensates form spatially inhomogeneous network fluids Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Furqan Dar, Samuel R. Cohen, Diana M. Mitrea, Aaron H. Phillips, Gergely Nagy, Wellington C. Leite, Christopher B. Stanley, Jeong-Mo Choi, Richard W. Kriwacki, Rohit V. Pappu
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A global meta-analysis on the effects of organic and inorganic fertilization on grasslands and croplands Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Ting-Shuai Shi, Scott L. Collins, Kailiang Yu, Josep Peñuelas, Jordi Sardans, Hailing Li, Jian-Sheng Ye
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LSD1 drives intestinal epithelial maturation and controls small intestinal immune cell composition independent of microbiota in a murine model Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Alberto Díez-Sánchez, Håvard T. Lindholm, Pia M. Vornewald, Jenny Ostrop, Rouan Yao, Andrew B. Single, Anne Marstad, Naveen Parmar, Tovah N. Shaw, Mara Martín-Alonso, Menno J. Oudhoff
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Prediction error processing and sharpening of expected information across the face-processing hierarchy Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Annika Garlichs, Helen Blank
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Atomic-scale visualization of the interlayer Rydberg exciton complex in moiré heterostructures Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Meng Zhao, Zhongjie Wang, Lu Liu, Chunzheng Wang, Cheng-Yen Liu, Fang Yang, Hua Wu, Chunlei Gao
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Double cross-linked 3D layered PBI proton exchange membranes for stable fuel cell performance above 200 °C Nat. Commun. (IF 16.6) Pub Date : 2024-04-22 Liang Zhang, Mengjiao Liu, Danyi Zhu, Mingyuan Tang, Taizhong Zhu, Congjie Gao, Fei Huang, Lixin Xue
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Harnessing the power of f-block elements in radiopharmaceuticals Nat. Rev. Chem. (IF 36.3) Pub Date : 2024-04-22 Alex Rigby, Trevor Arino
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Designer peptide–DNA cytoskeletons regulate the function of synthetic cells Nat. Chem. (IF 21.8) Pub Date : 2024-04-23 Margaret L. Daly, Kengo Nishi, Stephen J. Klawa, Kameryn Y. Hinton, Yuan Gao, Ronit Freeman
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India’s 50-year-old Chipko movement is a model for environmental activism Nature (IF 64.8) Pub Date : 2024-04-23
Letter to the Editor
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The Middle East’s largest hypersaline lake risks turning into an environmental disaster zone Nature (IF 64.8) Pub Date : 2024-04-23
Letter to the Editor
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Charles Darwin investigates: the curious case of primrose punishment Nature (IF 64.8) Pub Date : 2024-04-23
Snippets from Nature’s past.
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Chemistry lab destroyed by Taiwan earthquake has physical and mental impacts Nature (IF 64.8) Pub Date : 2024-04-23
Letter to the Editor
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More work is needed to take on the rural wastewater challenge Nature (IF 64.8) Pub Date : 2024-04-23
Letter to the Editor
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Any plan to make smoking obsolete is the right step Nature (IF 64.8) Pub Date : 2024-04-23
The United Kingdom is correct to attempt to end the single largest preventable cause of illness and death, as was New Zealand before its government changed its mind.
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European ruling linking climate change to human rights could be a game changer — here’s how Nature (IF 64.8) Pub Date : 2024-04-23
The European Court of Human Rights’ judgment in a Swiss case cements the concept that climate inaction violates human rights — responsible nations around the world will take heed.
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Lethal AI weapons are here: how can we control them? Nature (IF 64.8) Pub Date : 2024-04-23
Autonomous weapons guided by artificial intelligence are already in use. Researchers, legal experts and ethicists are struggling with what should be allowed on the battlefield.
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Star Formation Shut Down by Multiphase Gas Outflow in a Galaxy at a Redshift of 2.45 Nature (IF 64.8) Pub Date : 2024-04-22 Sirio Belli, Minjung Park, Rebecca L. Davies, J. Trevor Mendel, Benjamin D. Johnson, Charlie Conroy, Chloë Benton, Letizia Bugiani, Razieh Emami, Joel Leja, Yijia Li, Gabriel Maheson, Elijah P. Mathews, Rohan P. Naidu, Erica J. Nelson, Sandro Tacchella, Bryan A. Terrazas, Rainer Weinberger
Large-scale outflows driven by supermassive black holes are thought to play a fundamental role in suppressing star formation in massive galaxies. However, direct observational evidence for this hypothesis is still lacking, particularly in the young universe where star formation quenching is remarkably rapid1–3, thus requiring effective removal of gas4 as opposed to slow gas heating5,6. While outflows
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Dozens of genes are linked to post-traumatic stress disorder Nature (IF 64.8) Pub Date : 2024-04-22
Findings underscore that genetic factors contribute to development of the condition after a traumatic incident.
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Multimodal cell atlas of the ageing human skeletal muscle Nature (IF 64.8) Pub Date : 2024-04-22 Yiwei Lai, Ignacio Ramírez-Pardo, Joan Isern, Juan An, Eusebio Perdiguero, Antonio L. Serrano, Jinxiu Li, Esther García-Domínguez, Jessica Segalés, Pengcheng Guo, Vera Lukesova, Eva Andrés, Jing Zuo, Yue Yuan, Chuanyu Liu, José Viña, Julio Doménech-Fernández, Mari Carmen Gómez-Cabrera, Yancheng Song, Longqi Liu, Xun Xu, Pura Muñoz-Cánoves, Miguel A. Esteban
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Your perception of time is skewed by what you see Nature (IF 64.8) Pub Date : 2024-04-22
Features of a scene such as size and clutter can affect the brain’s sense of how much time has passed while observing it.
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Daily briefing: Great Barrier Reef is experiencing its worst mass bleaching event on record Nature (IF 64.8) Pub Date : 2024-04-22
Iconic coral reef is ‘transforming’ from repeated bleaching events. Plus, researchers face the possibility of animal consciousness and science explores the neurodiversity of visual imagery.
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How volcanoes shaped our planet — and why we need to be ready for the next big eruption Nature (IF 64.8) Pub Date : 2024-04-22
The world should learn from past disasters and prepare for the effects of future, inevitable volcanic catastrophes, a wide-reaching book teaches us.
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Daily briefing: why queasiness kills hunger Nature (IF 64.8) Pub Date : 2024-04-19
Feelings of hunger, nausea and fullness seem to be governed by separate brain circuits. Plus, nearly half of China’s major cities are sinking and Jupiter’s moon, Io, is the most volcanically active place in the Solar System.
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Daily briefing: ‘Goldene’ is a gilded cousin of graphene that is one atom thick Nature (IF 64.8) Pub Date : 2024-04-18
Single-atom-thick sheet of gold is probably the first 2D metal. Plus, some bumblebees can survive up to a week underwater and what crackdowns on smoking and vaping will do for public health.
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On the fundamentals of quantum rate theory and the long-range electron transport in respiratory chains Chem. Soc. Rev. (IF 46.2) Pub Date : 2024-04-23 Paulo Roberto Bueno
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Redox regulation of Ni hydroxides with controllable phase composition towards biomass-derived polyols electro-refinery Chem. Sci. (IF 8.4) Pub Date : 2024-04-23 Yi Tang, Zhuxin Gui, Yingshuai Jia, Xianping Liao, Tianlan Yan, Boxu Gao, Wenbiao Zhang, Li Chen, Qingsheng Gao, Yahong Zhang
Electrocatalytic refinery from biomass-derived glycerol (GLY) to formic acid (FA), one of the most promising candidates of green H2 carrier, has driven widespread attention for its sustainability. Herein, we fabricated a series of monolithic Ni hydroxides-based electrocatalysts by a facile and in-situ electrochemical method through the manipulation of local pH near electrode. The as-synthesized Ni(OH)2@NF-1
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Viologen-based solution-processable ionic porous polymers for electrochromic applications Chem. Sci. (IF 8.4) Pub Date : 2024-04-23 Hongya Miao, Ling Chen, Fangfang Xing, Huijie Li, Thomas Baumgartner, Xiaoming He
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Understanding Electrochemical Interfaces through Comparing Experimental and Computational Charge Density-Potential Curves Chem. Sci. (IF 8.4) Pub Date : 2024-04-23 Nandita Mohandas, Sumit Bawari, Jani J.T. Shibuya, Soumya Ghosh, Jagannath Mondal, Tharangattu N. Narayanan, Angel Cuesta
Electrode-electrolyte interfaces play a decisive role in electrochemical charge accumulation and transfer processes. Theoretical modelling of these interfaces is critical to decipher the microscopic details of such phenomena. Different force field-based molecular dynamics protocols are compared here in a view to connect calculated and experimental charge density-potential relationships. Platinum-aqueous
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Enantioselective synthesis of α-aryl α-hydrazino phosphonates Chem. Sci. (IF 8.4) Pub Date : 2024-04-23 Saul Alberca, Javier Romero-Parra, Israel Fernandez, Rosario Fernández, Jose M. Lassaletta, David Monge
Catalysts generated in situ by the combination of pyridine-hydrazone N,N-ligands and Pd(TFA)2 have been applied to the addition of arylboronic acids to formylphosphonate-derived hydrazones, yielding α-aryl α-hydrazino phosphonates in excellent enantioselectivities (96−>99% ee). Subsequent removal of the benzyloxycarbonyl (Cbz) N-protecting group afforded key building blocks en route to appealing artificial
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Monolithic 3D nanoelectrospray emitters based on continuous fluid-assisted etching strategy for glass droplet microfluidic chip-mass spectrometry Chem. Sci. (IF 8.4) Pub Date : 2024-04-23 Yaoyao Zhao, Ziyang Guo, Yingqi Zhao, Zhao Jin, Yaran Chang, Xiayan Wang, Guangsheng Guo
Glass microfluidic chips are suitable for coupling with mass spectrometry (MS) due to their flexible design, optical transparency and resistance to organic reagents. However, due to the high hardness and brittleness of glass, there is a lack of simple and feasible technology to manufacture a monolithic nanospray ionization (nESI) emitter on a glass microchip, which hinders its coupling with mass spectrometry
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Photo-Thermal Synergistic CO2 Hydrogenation towards CO over PtRh Bimetal-Decorated GaN Nanowires/Si Chem. Sci. (IF 8.4) Pub Date : 2024-04-23 Jinglin Li, Bowen Sheng, Liang Qiu, Jiajia Yang, Ping Wang, Yixin Li, Tianqi Yu, Hu Pan, Ying Li, Muhan Li, Lei Zhu, Xinqiang Wang, Zhen Huang, Baowen Zhou
Photo-thermal-synergistic hydrogenation is a promising strategy for upcycling carbon dioxide into fuels and chemicals by maximally utilizing full-spectrum solar energy. Herein, by immobilizing Pt-Rh bimetal onto a well-developed GaN NWs/Si platform, CO2 was photo-thermo-catalytically hydrogenated towards CO under concentrated light illumination without extra energies. The as-designed architecture demonstrates
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Optoelectronic insights of lead-free layered halide perovskites Chem. Sci. (IF 8.4) Pub Date : 2024-04-23 Vishwadeepa Hazra, Arnab Mandal, Sayan Bhattacharyya
Two-dimensional organic-inorganic halide perovskites have emerged as promising candidates for a multitude of optoelectronic technologies, owing to their versatile structure and electronic properties. The optical and electronic properties are harmoniously integrated with both the inorganic metal halide octahedral slab, and the organic spacer layer. The inorganic octahedral layers can also assemble into
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1,5-Hydrogen Atom Transfer of α-Iminyl Radical Cations: A New Platform for Relay Annulation towards Pyridine Derivatives and Axially Chiral Heterobiaryls Chem. Sci. (IF 8.4) Pub Date : 2024-04-23 Yu-Qiang Zhou, Kui-Cheng He, Wei-Hao Zheng, Jing-Fang Lv, Shi-Mei He, Ning Yu, Yun-Bo Yang, Lv-Yan Liu, Kun Jiang, Ye Wei
The exploitation of new reactive species and novel transformation modes for their synthetic applications have significantly promoted the development of synthetic organic methodology, drug discovery, and advanced functional materials. α-Iminyl radical cations, a class of distonic ions, exhibit great synthetic potential towards the synthesis of valuable molecules. For their generation, radical conjugate
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Highly intense NIR emissive Cu4Pt2 bimetallic clusters featuring Pt(I)-Cu4-Pt(I) sandwich kernel Chem. Sci. (IF 8.4) Pub Date : 2024-04-23 Rui-Ru Zhong, Mo Xie, Cui-Zhou Luan, Lin-Mei Zhang, De-Bo Hao, Shang-Fu Yuan, Tao Wu
Metal nanoclusters (NCs) capable of near-infrared (NIR) photoluminescence (PL) are gaining increasing interest for their potential applications in bioimaging, cell labelling, and phototherapy. However, the limited quantum yield (QY) of NIR emission in metal NCs, especially those emitting beyond 800 nm, hinders their widespread applications. Herein, we present a bright NIR luminescence (PLQY up to 36%