Direct access to N-alkylated amines and imines via acceptorless dehydrogenative coupling catalyzed by a cobalt(ii)-NNN pincer complex†,Catalysis Science & Technology

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Direct access to N-alkylated amines and imines via acceptorless dehydrogenative coupling catalyzed by a cobalt(ii)-NNN pincer complex†
Catalysis Science & Technology ( IF 5 ) Pub Date : 2018-06-22 00:00:00 , DOI: 10.1039/c8cy00859k
Siba P. Midya _{1,

2,

3,

4} , Jayaraman Pitchaimani _{4,

5,

6,

7} , Vinod G. Landge _{1,

2,

3,

4} , Vedichi Madhu _{4,

5,

6,

7} , Ekambaram Balaraman _{1,

2,

3,

4}

Affiliation

A simple, phosphine-free Co(II)-NNN pincer complex catalyzed direct N-alkylation of anilines with alcohols via hydrogen auto-transfer (HA) and selective acceptorless dehydrogenative coupling (ADC) of benzylamines with alcohols affording imines with the liberation of molecular hydrogen and water is reported.

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