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Proton-Conductor-Gated MoS2 Transistors with Room Temperature Electron Mobility of >100 cm2 V–1 s–1
Chemistry of Materials ( IF 8.6 ) Pub Date : 2018-06-19 00:00:00 , DOI: 10.1021/acs.chemmater.8b00568
Yongsuk Choi , Hyunwoo Kim , Jeehye Yang 1 , Seung Won Shin , Soong Ho Um , Sungjoo Lee , Moon Sung Kang 1 , Jeong Ho Cho
Affiliation  

Room temperature electron mobility of >100 cm2 V–1 s–1 is achieved for a few-layer MoS2 transistor by use of a polyanionic proton conductor as the top-gate dielectric of the device. The use of a proton conductor that inherently exhibits a cationic transport number close to 1 yields unipolar electron transport in the MoS2 channel. The high mobility value is attributed to the effective formation of an electric double layer by the proton conductor, which facilitates electron injection into the MoS2 channel, and to the effective screening of the charged impurities in the vicinity of the device channel. Through careful temperature-dependent transistor and capacitor measurements, we also confirm quenching of the phonon modes in the proton-conductor-gated MoS2 channel, which should also contribute to the achieved high mobility. These devices are then used to assemble a simple resistive-load inverter logic circuit, which can be switched at high frequencies above 1 kHz.

中文翻译:

质子导体门控的MoS 2晶体管,室温电子迁移率> 100 cm 2 V –1 s –1

通过使用聚阴离子质子导体作为器件的顶栅电介质,可对几层MoS 2晶体管实现室温电子迁移率> 100 cm 2 V –1 s –1。固有地表现出接近1的阳离子传输数的质子导体的使用会在MoS 2通道中产生单极电子传输。高迁移率值归因于质子导体有效地形成双电层,这有助于电子注入到MoS 2中通道,并有效筛选设备通道附近的带电杂质。通过仔细的温度相关晶体管和电容器测量,我们还确认了质子导体门控MoS 2通道中声子模的猝灭,这也应有助于实现高迁移率。然后,这些设备用于组装简单的电阻负载逆变器逻辑电路,该电路可以在高于1 kHz的高频下进行切换。
更新日期:2018-06-19
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