Electrochemical calcium extraction from 1D-Ca3Co2O6†,Dalton Transactions

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Electrochemical calcium extraction from 1D-Ca3Co2O6†
Dalton Transactions ( IF 4 ) Pub Date : 2018-06-14 00:00:00 , DOI: 10.1039/c8dt01754a
Deyana S. Tchitchekova _{1,

2,

3} , Carlos Frontera _{1,

2,

3} , Alexandre Ponrouch _{1,

2,

3} , Christopher Krich _{4,

5,

6,

7,

8} , Fanny Bardé _{4,

5,

6,

7,

8} , M. Rosa Palacín _{1,

2,

3}

Affiliation

The electrochemical oxidation of a transition metal oxide through calcium extraction is achieved for the first time. The 1D framework of Ca₃Co₂O₆ is maintained upon oxidation and the new phase formed exhibits a modulated structure. The process occurs at high potential and is partially reversible, which opens prospects for a calcium battery proof-of-concept.

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