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A Process for Capturing CO2 from the Atmosphere
Joule ( IF 39.8 ) Pub Date : 2018-06-07 , DOI: 10.1016/j.joule.2018.05.006
David W. Keith , Geoffrey Holmes , David St. Angelo , Kenton Heidel

We describe a process for capturing CO2 from the atmosphere in an industrial plant. The design captures ∼1 Mt-CO2/year in a continuous process using an aqueous KOH sorbent coupled to a calcium caustic recovery loop. We describe the design rationale, summarize performance of the major unit operations, and provide a capital cost breakdown developed with an independent consulting engineering firm. We report results from a pilot plant that provides data on performance of the major unit operations. We summarize the energy and material balance computed using an Aspen process simulation. When CO2 is delivered at 15 MPa, the design requires either 8.81 GJ of natural gas, or 5.25 GJ of gas and 366 kWhr of electricity, per ton of CO2 captured. Depending on financial assumptions, energy costs, and the specific choice of inputs and outputs, the levelized cost per ton CO2 captured from the atmosphere ranges from 94 to 232 $/t-CO2.



中文翻译:

从大气中捕获CO 2的过程

我们描述了一种在工厂中从大气中捕获CO 2的方法。该设计使用与钙苛性碱回收回路耦合的含水KOH吸附剂,在连续过程中每年捕获约1 Mt-CO 2。我们描述了设计原理,总结了主要部门运营的绩效,并提供了由独立咨询工程公司开发的资本成本明细表。我们报告了一家中试工厂的结果,该工厂提供了有关主要部门运营绩效的数据。我们总结了使用Aspen工艺仿真计算出的能量和材料平衡。当以15 MPa的压力输送CO 2时,该设计需要每吨CO 2消耗8.81 GJ天然气或5.25 GJ天然气和366 kWhr的电力被抓获。根据财务假设,能源成本以及投入和产出的特定选择,从大气中捕获的每吨CO 2的平均成本为94至232美元/吨CO 2

更新日期:2018-06-07
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