当前位置: X-MOL 学术Catal. Commun. › 论文详情
Our official English website, www.x-mol.net, welcomes your feedback! (Note: you will need to create a separate account there.)
Enhanced activity of TiO2 by concentrating light for photoreduction of CO2 with H2O to CH4
Catalysis Communications ( IF 3.7 ) Pub Date : 2018-05-10 , DOI: 10.1016/j.catcom.2018.05.005
Dong Li , Yinfei Chen , Stéphane Abanades , Zekai Zhang

Concentrating light technology is used to improve photoreduction of CO2 to CH4 reaction on semiconductor catalysts such as TiO2. The catalysts were prepared by anodization method and characterized by XRD, SEM, XPS and photoillumiation. The results showed that the CH4 yield rate could be raised from 0.70 μmol g−1 h−1 to 20.67 μmol g−1 h−1 under concentrating light, and it could be further increased to 28.49 μmol g−1 h−1 after pretreatment in the air. It is inferred that the concentrating light increases CO2 conversion not only by heightening light intensity, but also by improving the surface properties of the catalyst.



中文翻译:

通过聚集光以将H 2 O还原为CH 4的CO 2增强TiO 2的活性

聚光技术用于改善在半导体催化剂(如TiO 2)上将CO 2还原为CH 4的光还原能力。通过阳极氧化法制备了催化剂,并通过XRD,SEM,XPS和光致发光进行了表征。结果表明,在聚光条件下,CH 4的得率可以从0.70μmolg -1  h -1提高到20.67μmolg -1  h -1,经过进一步的提高,可以进一步提高到28.49μmolg -1  h -1。在空气中进行预处理。可以推测,聚光使CO 2增加 转化不仅通过提高光强度,而且还通过改善催化剂的表面性能。

更新日期:2018-05-10
down
wechat
bug