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On the performance optimisation of Fe catalysts in the microwave - assisted H2 production by the dehydrogenation of hexadecane
Catalysis Today ( IF 5.3 ) Pub Date : 2018-03-19 , DOI: 10.1016/j.cattod.2018.03.036
X. Jie , T. Xiao , B. Yao , S. Gonzalez-Cortes , J. Wang , Y. Fang , N. Miller , H. AlMegren , J.R. Dilworth , P.P. Edwards

Microwave - assisted catalysis has previously been shown to offer unique advantages in the rapid production of hydrogen from hydrocarbons fuels. In this work, we have prepared a series of supported catalysts with varying iron content and support materials, and evaluated the resulting H2 production from hexadecane, a key representative component of diesel fuel. These catalysts, under microwave activation, exhibit high selectivity for H2 over hydrocarbons in the effluent gas. Microwave-assisted Fe catalysts supported on SiC at low Fe loading levels (<10 wt.%) are found to be the most effective catalytic system for rapid and high-purity H2 production from hexadecane.



中文翻译:

十六烷脱氢微波辅助H 2生产中Fe催化剂的性能优化研究。

以前已经证明,微波辅助催化在从碳氢化合物燃料快速生产氢方面提供独特的优势。在这项工作中,我们准备了一系列具有不同铁含量和载体材料的负载型催化剂,并评估了由十六烷(柴油的关键代表成分)产生的H 2的产生。这些催化剂在微波活化下对废气中的烃显示出对H 2的高选择性。发现以低铁含量(<10 wt。%)负载在SiC上的微波辅助铁催化剂是从十六烷中快速,高纯度生产H 2的最有效的催化体系。

更新日期:2018-03-19
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