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Experimental Insights into Ground-State Selection of Quantum XY Pyrochlores
Annual Review of Condensed Matter Physics ( IF 22.6 ) Pub Date : 2018-03-12 00:00:00 , DOI: 10.1146/annurev-conmatphys-031016-025218
Alannah M. Hallas 1 , Jonathan Gaudet 1 , Bruce D. Gaulin 1, 2, 3
Affiliation  

Extensive experimental investigations of the magnetic structures and excitations in the XY pyrochlores have been carried out over the past decade. Three families of XY pyrochlores have emerged: Yb2B2O7, Er2B2O7, and, most recently, Co2F7. In each case, the magnetic cation (either Yb, Er, or Co) exhibits XY anisotropy within the local pyrochlore coordinates, a consequence of crystal field effects. Materials in these families display rich phase behavior and are candidates for exotic ground states, such as quantum spin ice, and exotic ground-state selection via order-by-disorder mechanisms. In this review, we present an experimental summary of the ground-state properties of the XY pyrochlores, including evidence that they are strongly influenced by phase competition. We empirically demonstrate the signatures for phase competition in a frustrated magnet: multiple heat capacity anomalies, suppressed TN or TC, sample- and pressure-dependent ground states, and unconventional spin dynamics.

中文翻译:


量子XY烧绿石基态选择的实验见解

在过去的十年中,对XY烧绿石中的磁性结构和激发进行了广泛的实验研究。出现了三个系列的XY烧绿石:Yb 2 B 2 O 7,Er 2 B 2 O 7,最近,Co 2 F 7。在每种情况下,磁阳离子(Yb,Er或Co)在局部烧绿石坐标内均表现出XY各向异性,这是晶体场效应的结果。这些族中的材料显示出丰富的相行为,并且是诸如量子自旋冰之类的奇异基态的候选者,以及通过逐序机制对奇异基态进行选择的材料。在这篇综述中,我们提供了XY烧绿石基态性质的实验总结,包括它们受相竞争强烈影响的证据。我们凭经验证明了沮丧的磁体中相竞争的特征:多重热容量异常,抑制的T NT C,取决于样品和压力的基态以及非常规的自旋动力学。

更新日期:2018-03-12
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