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Constructing interfacial contact for enhanced photocatalytic activity through BiOIO3/g-C3N4 nanoflake heterostructure
Catalysis Communications ( IF 3.7 ) Pub Date : 2018-02-26 , DOI: 10.1016/j.catcom.2018.02.018
Jiang Wu , Pengfei Sheng , Weixing Xu , Xiao Zhou , Cheng Lu , Zheng Ji , Kai Xu , Liangjun Zhu , Xia Zhang , Wei Feng

The highly efficient BiOIO3/g-C3N4 with unique nanoflake heterostructures were synthesized through hydrothermal method by simply depositing BiOIO3 flake on the surface of g-C3N4. Photocatalytic ability of nanoflakes was tested by oxidation of gaseous Hg0 under 18 W and 24 W LED light irradiation. The g-C3N4/BiOIO3 composite with the molar ratio of 10:1 exhibited that the Hg0 removal efficiency reached up to 93.7%. The remarkable photocatalytic performance of the as-prepared catalysts can be attributed to the interfacial contact heterostructure formed between BiOIO3 and g-C3N4, which constructs an intimate interfacial interaction between the two components. Moreover, well-matched band structure can efficiently lead to the separation of photogenerated charges.



中文翻译:

通过BiOIO 3 / gC 3 N 4纳米片异质结构构建界面接触以增强光催化活性

高效BiOIO 3 / GC 3 Ñ 4具有独特的纳米片的异质结构是通过水热法通过简单地沉积BiOIO合成3的GC表面薄片3 Ñ 4。通过在18 W和24 W LED光照射下气态Hg 0的氧化测试了纳米薄片的光催化能力。摩尔比为10:1的gC 3 N 4 / BiOIO 3复合材料表现出Hg 0去除效率达到93.7%。所制备的催化剂具有显着的光催化性能,这可以归因于BiOIO 3和gC 3 N 4之间形成的界面接触异质结构,这在两种组分之间建立了紧密的界面相互作用。而且,良好匹配的能带结构可以有效地导致光生电荷的分离。

更新日期:2018-02-26
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