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2D Black Phosphorus: from Preparation to Applications for Electrochemical Energy Storage
Advanced Science ( IF 15.1 ) Pub Date : 2018-02-23 , DOI: 10.1002/advs.201700491
Shuxing Wu 1 , Kwan San Hui 2 , Kwun Nam Hui 1
Affiliation  

Black phosphorus (BP) is rediscovered as a 2D layered material. Since its first isolation in 2014, 2D BP has triggered tremendous interest in the fields of condensed matter physics, chemistry, and materials science. Given its unique puckered monolayer geometry, 2D BP displays many unprecedented properties and is being explored for use in numerous applications. The flexibility, large surface area, and good electric conductivity of 2D BP make it a promising electrode material for electrochemical energy storage devices (EESDs). Here, the experimental and theoretical progress of 2D BP is presented on the basis of its preparation methods. The structural and physiochemical properties, air instability, passivation, and EESD applications of 2D BP are discussed systemically. Specifically, the latest research findings on utilizing 2D BP in EESDs, such as lithium‐ion batteries, supercapacitors, and emerging technologies (lithium–sulfur batteries, magnesium‐ion batteries, and sodium‐ion batteries), are summarized. On the basis of the current progress, a few personal perspectives on the existing challenges and future research directions in this developing field are provided.

中文翻译:

二维黑磷:从电化学储能的制备到应用

黑磷 (BP) 作为一种二维层状材料被重新发现。自 2014 年首次分离以来,2D BP 引发了凝聚态物理、化学和材料科学领域的巨大兴趣。鉴于其独特的褶皱单层几何形状,2D BP 显示出许多前所未有的特性,并正在探索在众多应用中的使用。2D BP 的柔韧性、大比表面积和良好的导电性使其成为电化学储能器件(EESD)的有前途的电极材料。在此,根据其制备方法介绍了二维BP的实验和理论进展。系统地讨论了 2D BP 的结构和理化性质、空气不稳定性、钝化和 EESD 应用。具体来说,总结了在锂离子电池、超级电容器和新兴技术(锂硫电池、镁离子电池和钠离子电池)等EESD中利用2D BP的最新研究成果。在当前进展的基础上,对该发展领域现有的挑战和未来的研究方向提出了一些个人观点。
更新日期:2018-02-23
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