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TiO2 on MoSe2 nanosheets as an advanced photocatalyst for hydrogen evolution in visible light
Catalysis Communications ( IF 3.7 ) Pub Date : 2017-12-24 , DOI: 10.1016/j.catcom.2017.12.013
Shufang Kou , Xia Guo , Xiaofeng Xu , Jian Yang

TiO2 grown on MoSe2 nanosheets was synthesized by a simple process and explored as photocatalyst for hydrogen generation. In visible light, hydrogen generation rate over the MoSe2/TiO2 photocatalyst was found to be 468.2 μmol h− 1 g− 1, much higher than the corresponding rates obtained over the MoSe2, TiO2 and their physical mixture. It is suggested that the good absorption of MoSe2 to visible light and the improved charge separation by the interface of MoSe2/TiO2 greatly promote hydrogen generation rate, as supported by the transient photocurrent responses and electrochemical impedance spectra recorded.



中文翻译:

MoSe 2纳米片上的TiO 2作为先进的光催化剂,用于在可见光中析氢

通过简单的方法合成了在MoSe 2纳米片上生长的TiO 2,并将其作为光催化剂用于制氢。在可见光下,发现在MoSe 2 / TiO 2光催化剂上的氢气产生速率为468.2μmolh -1  g -1,远高于在MoSe 2 / TiO 2及其物理混合物上获得的相应速率。这表明MoSe 2对可见光的良好吸收和通过MoSe 2 / TiO 2的界面改善的电荷分离 通过记录的瞬态光电流响应和电化学阻抗谱,大大提高了氢气的产生速率。

更新日期:2017-12-24
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