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One-Step Reforming of CO2 and CH4 into High-Value Liquid Chemicals and Fuels at Room Temperature by Plasma-Driven Catalysis
Angewandte Chemie International Edition ( IF 16.6 ) Pub Date : 2017-09-19 08:10:27 , DOI: 10.1002/anie.201707131
Li Wang 1 , Yanhui Yi 2 , Chunfei Wu 3 , Hongchen Guo 2 , Xin Tu 1
Affiliation  

Liquid fuels and chemicals (e.g., acetic acid, methanol, ethanol, and formaldehyde) were synthesized in a one-step process from CO2 and CH4 at room temperature (30 °C) and atmospheric pressure for the first time by using a novel plasma reactor with a water electrode. The total selectivity to oxygenates was approximately 50–60 %, with acetic acid as the major component.

中文翻译:

等离子体驱动催化在室温下一步一步将CO2和CH4重整为高价值液体化学品和燃料

通过使用新颖的方法,首次在室温(30°C)和大气压下由CO 2和CH 4一步一步合成液体燃料和化学品(例如,乙酸,甲醇,乙醇和甲醛)带有水电极的等离子体反应器。以乙酸为主要成分,对含氧化合物的总选择性约为50-60%。
更新日期:2017-09-19
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